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公开(公告)号：US08226896B2
公开(公告)日：2012-07-24
申请号：US12525678
申请日：2008-01-28
申请人： Marcus Pfeifer , Markus Koegel , Wolfgang Schneider , Nicola Soeger , Katja Adelmann , Gerald Jeske , Thomas Kreuzer
发明人： Marcus Pfeifer , Markus Koegel , Wolfgang Schneider , Nicola Soeger , Katja Adelmann , Gerald Jeske , Thomas Kreuzer
IPC分类号： B01D50/00
CPC分类号： F01N3/0814 , B01D53/9418 , B01D53/944 , B01D53/9468 , B01D2255/1021 , B01D2255/1023 , B01D2255/20738 , B01D2255/20761 , B01D2255/502 , B01D2255/9022 , B01D2258/012 , B01J23/40 , B01J23/63 , B01J29/106 , B01J29/24 , B01J29/46 , B01J29/7615 , B01J35/0006 , B01J37/0244 , F01N3/035 , F01N3/0821 , F01N3/0828 , F01N3/0842 , F01N3/2066 , F01N2240/25 , F01N2570/18 , F01N2610/02 , Y02T10/22 , Y02T10/24
摘要： A catalytically active diesel particulate filter with ammonia trap action is presented, which, in addition to an oxidation-active coating (2), comprises a coating (1) which is catalytically active in the SCR reaction. By means of this inventive diesel particulate filter, it is possible to make exhaust gas aftertreatment systems for removing nitrogen oxides and particulates from the exhaust gas of lean engines considerably simpler and less expensive.
摘要翻译： 提出了具有氨捕集作用的催化活性柴油微粒过滤器，除了氧化活性涂层（2）外，还包括在SCR反应中具有催化活性的涂层（1）。 通过本发明的柴油微粒过滤器，可以制备用于从贫燃机的废气中除去氮氧化物和颗粒物的废气后处理系统更简单且更便宜。
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公开(公告)号：US20100058746A1
公开(公告)日：2010-03-11
申请号：US12525678
申请日：2008-01-28
申请人： Marcus Pfeifer , Markus Koegel , Wolfgang Schneider , Nicola Soeger , Katja Adelmann , Gerald Jeske , Thomas Kreuzer
发明人： Marcus Pfeifer , Markus Koegel , Wolfgang Schneider , Nicola Soeger , Katja Adelmann , Gerald Jeske , Thomas Kreuzer
CPC分类号： F01N3/0814 , B01D53/9418 , B01D53/944 , B01D53/9468 , B01D2255/1021 , B01D2255/1023 , B01D2255/20738 , B01D2255/20761 , B01D2255/502 , B01D2255/9022 , B01D2258/012 , B01J23/40 , B01J23/63 , B01J29/106 , B01J29/24 , B01J29/46 , B01J29/7615 , B01J35/0006 , B01J37/0244 , F01N3/035 , F01N3/0821 , F01N3/0828 , F01N3/0842 , F01N3/2066 , F01N2240/25 , F01N2570/18 , F01N2610/02 , Y02T10/22 , Y02T10/24
摘要： A catalytically active diesel particulate filter with ammonia trap action is presented, which, in addition to an oxidation-active coating (2), comprises a coating (1) which is catalytically active in the SCR reaction. By means of this inventive diesel particulate filter, it is possible to make exhaust gas aftertreatment systems for removing nitrogen oxides and particulates from the exhaust gas of lean engines considerably simpler and less expensive.
摘要翻译： 提出了具有氨捕集作用的催化活性柴油微粒过滤器，除了氧化活性涂层（2）外，还包括在SCR反应中具有催化活性的涂层（1）。 通过本发明的柴油微粒过滤器，可以制备用于从贫燃机的废气中除去氮氧化物和颗粒物的废气后处理系统更简单且更便宜。
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3.发明申请EXHAUST GAS PURIFICATION SYSTEM FOR THE TREATMENT OF ENGINE EXHAUST GASES BY MEANS OF SCR CATALYST 有权通过SCR催化剂处理发动机排气的排气净化系统公开(公告)号：US20110146237A1
公开(公告)日：2011-06-23
申请号：US12937089
申请日：2009-03-18
申请人： Katja Adelmann , Nicola Soeger , Marcus Pfeifer , Wolfgang Schneider , Gerald Jeske , Thomas Kreuzer
发明人： Katja Adelmann , Nicola Soeger , Marcus Pfeifer , Wolfgang Schneider , Gerald Jeske , Thomas Kreuzer
CPC分类号： B01D53/9418 , B01D53/9477 , B01D2255/20761 , B01D2255/20776 , B01D2255/407 , B01D2255/50 , B01D2258/012 , B01J23/002 , B01J23/30 , B01J29/072 , B01J29/7615 , B01J35/0006 , B01J37/0201 , B01J37/0246 , B01J37/0248 , B01J2523/00 , F01N3/035 , F01N3/106 , F01N3/2066 , F01N13/0093 , F01N2510/0682 , F01N2570/18 , Y02T10/24 , B01J2523/3712 , B01J2523/48
摘要： An exhaust gas purification system (method and device) for the treatment of diesel exhaust gases containing nitrogen oxides and hydrocarbons is disclosed, which comprises the addition of ammonia or of a compound decomposable to ammonia into the exhaust gas stream and the subsequent leading of the exhaust gas stream over two successively arranged SCR catalysts with different properties and compositions. Both SCR catalysts are free of vanadium compounds and only the downstream SCR catalyst contains zeolite compounds. The exhaust gas purification system according to the invention is characterized by good “kick-off” behavior at low temperatures and a simultaneously high conversion performance over a wide temperature range.
摘要翻译： 公开了一种用于处理含有氮氧化物和烃的柴油废气的废气净化系统（方法和装置），其包括将氨或可分解成氨的化合物加入排气流中，随后引导排气 气流在两个连续排列的SCR催化剂上具有不同的性能和组成。 两种SCR催化剂都不含钒化合物，只有下游SCR催化剂含有沸石化合物。 根据本发明的废气净化系统的特征在于在低温下具有良好的“启动”行为，并且在宽的温度范围内具有同时高的转换性能。
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4.发明授权Exhaust gas purification system for the treatment of engine exhaust gases by means of SCR catalyst 有权用于通过SCR催化剂处理发动机废气的废气净化系统公开(公告)号：US08863507B2
公开(公告)日：2014-10-21
申请号：US12937089
申请日：2009-03-18
申请人： Katja Adelmann , Nicola Soeger , Marcus Pfeifer , Wolfgang Schneider , Gerald Jeske , Thomas Kreuzer
发明人： Katja Adelmann , Nicola Soeger , Marcus Pfeifer , Wolfgang Schneider , Gerald Jeske , Thomas Kreuzer
IPC分类号： F01N3/10 , B01J23/00 , B01J29/76 , F01N3/20 , B01J35/00 , F01N13/00 , B01J23/30 , B01D53/94 , F01N3/035 , B01J37/02 , B01J29/072
CPC分类号： B01D53/9418 , B01D53/9477 , B01D2255/20761 , B01D2255/20776 , B01D2255/407 , B01D2255/50 , B01D2258/012 , B01J23/002 , B01J23/30 , B01J29/072 , B01J29/7615 , B01J35/0006 , B01J37/0201 , B01J37/0246 , B01J37/0248 , B01J2523/00 , F01N3/035 , F01N3/106 , F01N3/2066 , F01N13/0093 , F01N2510/0682 , F01N2570/18 , Y02T10/24 , B01J2523/3712 , B01J2523/48
摘要： An exhaust gas purification system (method and device) for the treatment of diesel exhaust gases containing nitrogen oxides and hydrocarbons is disclosed, which comprises the addition of ammonia or of a compound decomposable to ammonia into the exhaust gas stream and the subsequent leading of the exhaust gas stream over two successively arranged SCR catalysts with different properties and compositions. Both SCR catalysts are free of vanadium compounds and only the downstream SCR catalyst contains zeolite compounds. The exhaust gas purification system according to the invention is characterized by good “kick-off” behavior at low temperatures and a simultaneously high conversion performance over a wide temperature range.
摘要翻译： 公开了一种用于处理含有氮氧化物和烃的柴油废气的废气净化系统（方法和装置），其包括将氨或可分解成氨的化合物加入排气流中，随后引导排气 气流在两个连续排列的SCR催化剂上具有不同的性能和组成。 两种SCR催化剂都不含钒化合物，只有下游SCR催化剂含有沸石化合物。 根据本发明的废气净化系统的特征在于在低温下具有良好的“启动”行为，并且在宽的温度范围内具有同时高的转换性能。
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5.发明授权Vanadium-free catalyst for selective catalytic reduction and process for it's preparation 有权用于选择性催化还原的无钒催化剂及其制备方法公开(公告)号：US08569199B2
公开(公告)日：2013-10-29
申请号：US12444312
申请日：2007-09-17
申请人： Katja Adelmann , Nicola Soeger , Lothar Mussmann , Marcus Pfeifer , Gerald Jeske
发明人： Katja Adelmann , Nicola Soeger , Lothar Mussmann , Marcus Pfeifer , Gerald Jeske
CPC分类号： B01J23/002 , B01D53/9418 , B01D2251/2062 , B01D2255/2063 , B01D2255/20769 , B01D2255/20776 , B01D2255/20784 , B01D2255/407 , B01D2255/9155 , B01J23/10 , B01J23/24 , B01J23/30 , B01J23/888 , B01J27/04 , B01J37/0201 , B01J37/0248 , B01J2523/00 , B01J2523/3706 , B01J2523/3712 , B01J2523/48 , Y02A50/2325 , Y02T10/24 , B01J2523/69 , B01J2523/842
摘要： Selective catalytic reduction with ammonia or a compound that decomposes to ammonia is a known method for the removal of nitrogen oxides from the exhaust gas of primarily lean-burn internal combustion engines. The vanadium-containing SCR catalysts that have long been generally used for this are characterized by a good conversion profile. However, the volatility of vanadium oxide can, at higher exhaust gas temperatures, lead to the emission of toxic vanadium compounds. Zeolite-based SCR catalysts, which are used in particular in discontinuous SCR systems, constitute a very cost-intensive solution for the problem.A method is proposed by which a homogeneous cerium-zirconium mixed oxide is activated for the SCR reaction in a defined manner by the introduction of sulphur and/or transition metal. Using this method, a highly active, ageing-resistant SCR catalyst is provided, which represents a vanadium-free, cost-effective and high-performance alternative to the existing SCR catalysts and is suitable in particular for use in motor vehicles.
摘要翻译： 用氨或分解成氨的化合物进行选择性催化还原是从主要贫燃内燃机的废气中除去氮氧化物的已知方法。 长期以来一般使用的含钒SCR催化剂的特征在于良好的转化率。 然而，在更高的废气温度下，氧化钒的挥发性会导致有毒的钒化合物的排放。 特别是在不连续SCR系统中使用的基于沸石的SCR催化剂构成了该问题的非常成本高的解决方案。 提出了一种通过引入硫和/或过渡金属以规定的方式使均相铈锆混合氧化物活化用于SCR反应的方法。 使用这种方法，提供了高活性，耐老化的SCR催化剂，其代表了现有SCR催化剂的无钒，成本效益和高性能替代物，并且特别适用于机动车辆。
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6.发明申请VANADIUM-FREE CATALYST FOR SELECTIVE CATALYTIC REDUCTION AND PROCESS FOR IT'S PREPARATION 有权用于选择性催化还原的无钒催化剂及其制备方法公开(公告)号：US20100034717A1
公开(公告)日：2010-02-11
申请号：US12444312
申请日：2007-09-17
申请人： Katja Adelmann , Nicola Soeger , Lothar Mussmann , Marcus Pfeifer , Gerald Jeske
发明人： Katja Adelmann , Nicola Soeger , Lothar Mussmann , Marcus Pfeifer , Gerald Jeske
IPC分类号： B01D53/94 , B01J23/10 , B01J27/02 , B01J27/051 , B01J27/047 , B01J27/045 , B01J27/043 , B01D53/56
CPC分类号： B01J23/002 , B01D53/9418 , B01D2251/2062 , B01D2255/2063 , B01D2255/20769 , B01D2255/20776 , B01D2255/20784 , B01D2255/407 , B01D2255/9155 , B01J23/10 , B01J23/24 , B01J23/30 , B01J23/888 , B01J27/04 , B01J37/0201 , B01J37/0248 , B01J2523/00 , B01J2523/3706 , B01J2523/3712 , B01J2523/48 , Y02A50/2325 , Y02T10/24 , B01J2523/69 , B01J2523/842
摘要： Selective catalytic reduction with ammonia or a compound that decomposes to ammonia is a known method for the removal of nitrogen oxides from the exhaust gas of primarily lean-burn internal combustion engines. The vanadium-containing SCR catalysts that have long been generally used for this are characterized by a good conversion profile. However, the volatility of vanadium oxide can, at higher exhaust gas temperatures, lead to the emission of toxic vanadium compounds. Zeolite-based SCR catalysts, which are used in particular in discontinuous SCR systems, constitute a very cost-intensive solution for the problem.A method is proposed by which a homogeneous cerium-zirconium mixed oxide is activated for the SCR reaction in a defined manner by the introduction of sulphur and/or transition metal. Using this method, a highly active, ageing-resistant SCR catalyst is provided, which represents a vanadium-free, cost-effective and high-performance alternative to the existing SCR catalysts and is suitable in particular for use in motor vehicles.
摘要翻译： 用氨或分解成氨的化合物进行选择性催化还原是从主要贫燃内燃机的废气中除去氮氧化物的已知方法。 长期以来一般使用的含钒SCR催化剂的特征在于良好的转化率。 然而，在更高的废气温度下，氧化钒的挥发性会导致有毒的钒化合物的排放。 特别是在不连续SCR系统中使用的基于沸石的SCR催化剂构成了该问题的非常成本高的解决方案。 提出了一种通过引入硫和/或过渡金属以规定的方式使均相铈锆混合氧化物活化用于SCR反应的方法。 使用这种方法，提供了高活性，耐老化的SCR催化剂，其代表了现有SCR催化剂的无钒，成本效益和高性能替代物，并且特别适用于机动车辆。
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7.发明授权Catalytically coated diesel particle filter, process for producing it and its use 有权催化涂层柴油颗粒过滤器，生产过程及其应用公开(公告)号：US07922987B2
公开(公告)日：2011-04-12
申请号：US12377753
申请日：2007-08-17
申请人： Markus Koegel , Marcus Pfeifer , Gerald Jeske , Frank Walter Schuetze , Stéphanie Frantz , Thomas Kreuzer
发明人： Markus Koegel , Marcus Pfeifer , Gerald Jeske , Frank Walter Schuetze , Stéphanie Frantz , Thomas Kreuzer
CPC分类号： F01N3/035 , B01D53/944 , B01D2255/102 , B01D2255/206 , B01D2255/20738 , B01D2255/20761 , B01D2255/50 , B01D2255/912 , B01D2255/9155 , B01J23/44 , B01J29/126 , B01J29/7415 , B01J29/80 , B01J35/0006 , B01J37/0244 , B01J37/0246 , B01J37/0248 , F01N3/0222 , F01N3/0821 , F01N3/0835 , F01N2370/02 , F01N2370/04 , F01N2510/063 , F01N2510/0682 , Y02A50/2341 , Y10S502/514
摘要： A diesel particulate filter with an oxidation catalyst comprising platinum and palladium deposited thereon is described. Addition of HC storage components to the oxidation catalyst allows the conversion of hydrocarbons and carbon monoxide to be improved significantly.
摘要翻译： 描述了具有沉积在其上的铂和钯的氧化催化剂的柴油微粒过滤器。 将HC储存组分添加到氧化催化剂允许烃和一氧化碳的转化显着改善。
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8.发明申请CATALYTICALLY COATED DIESEL PARTICLE FILTER, PROCESS FOR PRODUCING IT AND ITS USE 有权催化涂层柴油颗粒过滤器，生产工艺及其使用过程公开(公告)号：US20100092358A1
公开(公告)日：2010-04-15
申请号：US12377753
申请日：2007-08-17
申请人： Markus Koegel , Marcus Pfeifer , Gerald Jeske , Frank Walter Schuetze , Stéphanie Frantz , Thomas Kreuzer
发明人： Markus Koegel , Marcus Pfeifer , Gerald Jeske , Frank Walter Schuetze , Stéphanie Frantz , Thomas Kreuzer
CPC分类号： F01N3/035 , B01D53/944 , B01D2255/102 , B01D2255/206 , B01D2255/20738 , B01D2255/20761 , B01D2255/50 , B01D2255/912 , B01D2255/9155 , B01J23/44 , B01J29/126 , B01J29/7415 , B01J29/80 , B01J35/0006 , B01J37/0244 , B01J37/0246 , B01J37/0248 , F01N3/0222 , F01N3/0821 , F01N3/0835 , F01N2370/02 , F01N2370/04 , F01N2510/063 , F01N2510/0682 , Y02A50/2341 , Y10S502/514
摘要： A diesel particulate filter with an oxidation catalyst comprising platinum and palladium deposited thereon is described. Addition of HC storage components to the oxidation catalyst allows the conversion of hydrocarbons and carbon monoxide to be improved significantly.
摘要翻译： 描述了具有沉积在其上的铂和钯的氧化催化剂的柴油微粒过滤器。 将HC储存组分添加到氧化催化剂允许烃和一氧化碳的转化显着改善。
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9.发明申请SELECTIVE CATALYTIC REDUCTION OF NITROGEN OXIDES IN THE EXHAUST GAS OF DIESEL ENGINES 审中-公开柴油发动机排气中氮氧化物的选择性催化还原公开(公告)号：US20110142737A1
公开(公告)日：2011-06-16
申请号：US12964394
申请日：2010-12-09
申请人： Michael SEYLER , Nicola Soeger , Katja Adelmann , Anke Schuler , Thomas R. Pauly , Gerald Jeske
发明人： Michael SEYLER , Nicola Soeger , Katja Adelmann , Anke Schuler , Thomas R. Pauly , Gerald Jeske
CPC分类号： B01D53/9418 , B01D2251/2062 , B01D2255/2065 , B01D2255/20761 , B01D2255/407 , B01D2255/50 , B01J23/10 , B01J29/072 , B01J29/7615 , B01J29/763 , B01J29/84 , B01J29/85 , B01J37/0246 , Y02T10/24
摘要： A catalyst and a process for selective catalytic reduction of nitrogen oxides in diesel engine exhaust gases with ammonia or a compound decomposable to ammonia are described. The exhaust gas to be cleaned is passed together with ammonia or a compound decomposable to ammonia over a catalyst which comprises a zeolite or a zeolite-like compound containing 1-10% by weight of copper, based on the total weight of the zeolite or of the zeolite-like compound, and a homogeneous cerium-zirconium mixed oxide and/or a cerium oxide. The zeolite used or the zeolite-like compound used is selected from the group consisting of chabazite, SAPO-34, ALPO-34 and zeolite-β.
摘要翻译： 描述了用氨或可分解成氨的化合物来选择性催化还原柴油机废气中的氮氧化物的催化剂和方法。 待清洗的废气与氨或可分解氨的化合物一起通过催化剂一起通过催化剂，该催化剂包含基于沸石的总重量或含有1-10重量％铜的沸石或类似化合物的沸石或基于 沸石状化合物和均匀的铈 - 锆混合氧化物和/或氧化铈。 所使用的沸石或使用的沸石样化合物选自菱沸石，SAPO-34，ALPO-34和沸石 - bgr。
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公开(公告)号：US08926925B2
公开(公告)日：2015-01-06
申请号：US14002581
申请日：2012-03-01
申请人： Nicola Soeger , Katja Adelmann , Michael Seyler , Thomas R. Pauly , Gerald Jeske
发明人： Nicola Soeger , Katja Adelmann , Michael Seyler , Thomas R. Pauly , Gerald Jeske
IPC分类号： B01D53/94 , F01N3/28 , B01J29/00 , B01J29/12 , B01J37/02 , B01J29/068 , B01J29/072 , B01J29/076 , B01J29/76 , B01J29/80 , B01J33/00 , B01J35/02 , B01J29/18 , B01J29/46 , B01J29/78 , F01N3/20 , B01J29/65
CPC分类号： B01J29/126 , B01D53/9418 , B01D2251/2062 , B01D2255/206 , B01D2255/50 , B01D2255/9022 , B01D2255/9205 , B01D2258/012 , B01J29/068 , B01J29/072 , B01J29/076 , B01J29/185 , B01J29/46 , B01J29/65 , B01J29/7615 , B01J29/7838 , B01J29/80 , B01J33/00 , B01J35/023 , B01J37/0244 , B01J37/0246 , F01N3/2066 , F01N2610/02 , Y02T10/24 , Y10S502/52712
摘要： A catalyst for the selective catalytic reduction of nitrogen oxides in diesel engine exhaust gases using ammonia or a precursor compound decomposable to ammonia. The catalyst includes two superposed coatings applied to a support body, of which the first coating applied directly to the support body includes a transition metal-exchanged zeolite and/or a transition metal-exchanged zeolite-like compound, and effectively catalyzes the SCR reaction. The second coating is applied to the first coating to cover it on the exhaust gas side and prevent hydrocarbons having at least three carbon atoms present in the exhaust gas from contacting the first coating, without blocking the passage of nitrogen oxides and ammonia to the first coating. The second coating may be formed from small-pore zeolites and/or small-pore, zeolite-like compounds, and from suitable oxides, especially silicon dioxide, germanium dioxide, aluminum oxide, titanium dioxide, tin oxide, cerium oxide, zirconium dioxide and mixtures thereof.
摘要翻译： 使用氨或可分解成氨的前体化合物选择性催化还原柴油机废气中的氮氧化物的催化剂。 催化剂包括施加到支撑体上的两个重叠的涂层，其中直接施加到支撑体上的第一涂层包括过渡金属交换的沸石和/或过渡金属交换的沸石样化合物，并有效地催化SCR反应。 将第二涂层施加到第一涂层以将其覆盖在废气侧，并且防止排气中存在的具有至少三个碳原子的烃与第一涂层接触，而不阻挡氮氧化物和氨到第一涂层 。 第二涂层可以由小孔沸石和/或小孔沸石类化合物和适合的氧化物，特别是二氧化硅，二氧化锗，氧化铝，二氧化钛，氧化锡，氧化铈，二氧化锆和 其混合物。
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