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    Silico-crystal method of preparing same and catalytic conversion therewith
    35.
    发明授权
    Silico-crystal method of preparing same and catalytic conversion therewith 失效
    制备其的硅溶胶法及其催化转化

    公开(公告)号：US4397827A

    公开(公告)日：1983-08-09

    申请号：US303276

    申请日：1981-09-17

    Applicant: Pochen Chu

    Inventor： Pochen Chu

    IPC: B01J29/70 ,  C01B37/02 ,  C01B39/48 ,  C01B33/20 ,  C01B33/28

    CPC classification number: B01J29/703 ,  C01B37/02 ,  C01B39/48

    Abstract: A new porous silico-crystal, designated as ZSM-48, a method of making same and the use thereof in catalytic conversion of organic compounds. The new product has a composition, expressed in terms of moles of anhydrous oxides per 100 moles of silica as follows:(0.05 to 5) N.sub.2 O: (0.1 to 10)M.sub.2 /.sub.n O: (0 to 4)Al.sub.2 O.sub.3 : (100)SiO.sub.2wherein M is at least one cation having a valence n, N is a mixture of C.sub.2 -C.sub.12 alkylamine and more preferably of C.sub.3 -C.sub.5 tetramethyl ammonium compound, and wherein the zeolite is characterized by the distinctive X-ray powder diffraction pattern shown in Table I.

    Abstract translation: 称为ZSM-48的新的多孔硅晶体，其制备方法及其在有机化合物的催化转化中的用途。 （0.05〜5）N2O：（0.1〜10）M2 / nO：（0〜4）Al2O3：（100）SiO2 其中M是至少一个具有n价的阳离子，N是C 2 -C 12烷基胺和更优选C 3 -C 5四甲基铵化合物的混合物，其中沸石的特征在于表中所示的独特的X射线粉末衍射图 一世。

    Aromatization process utilizing a pillared layered silicate plus a base metal or noble metal
    36.
    发明授权
    Aromatization process utilizing a pillared layered silicate plus a base metal or noble metal 失效
    使用柱状分层硅酸盐加贱金属或贵金属的芳构化方法

    公开(公告)号：US5008481A

    公开(公告)日：1991-04-16

    申请号：US459212

    申请日：1989-12-29

    Applicant: Ivy D. Johnson ,  Pochen Chu ,  Charles T. Kresge

    Inventor： Ivy D. Johnson ,  Pochen Chu ,  Charles T. Kresge

    IPC: C07C5/367 ,  C07C5/41

    CPC classification number: C07C5/415 ,  C07C5/367 ,  C07C5/417

    Abstract: There is provided a process for the aromatization of non-aromatic hydrocarbons having at least six carbon atoms. The non-aromatic feed is contacted with a catalyst which includes a base metal or noble metal which is incorporated into or onto a pillared layered silicate. A preferred pillared layered silicate is kenyaite containing interspathic silica, and a preferred base metal or noble metal is chromium.

    Abstract translation: 提供了一种使具有至少6个碳原子的非芳族烃芳构化的方法。 非芳族进料与催化剂接触，催化剂包括引入到柱状层状硅酸盐中或其上的贱金属或贵金属。 优选的柱状层状硅酸盐是含有间隙二氧化硅的肯尼亚，优选的贱金属或贵金属是铬。

    Zeolite catalyst composition and synthesis method
    38.
    发明授权
    Zeolite catalyst composition and synthesis method 失效
    沸石催化剂组成及合成方法

    公开(公告)号：US4868146A

    公开(公告)日：1989-09-19

    申请号：US236414

    申请日：1988-08-25

    Applicant: Pochen Chu ,  Albert B. Schwartz

    Inventor： Pochen Chu ,  Albert B. Schwartz

    IPC: B01J29/40 ,  B01J29/90 ,  C07C2/12 ,  C10G50/00

    CPC classification number: C10G50/00 ,  B01J29/40 ,  B01J29/90 ,  C07C2/12 ,  B01J2229/123 ,  B01J2229/16 ,  B01J2229/32 ,  C07C2529/40 ,  C07C2529/70 ,  Y02P20/584

    Abstract: A surface-inactive shape selective metallosilicate catalyst, useful for the conversion of lower molecular weight olefins to liquid hydrocarbons such as gasoline, distillate, and high viscosity lube oils, is prepared by forming a silica shell on a medium pore metallosilicate core by crystallizing silica in the presence of fluoride ion onto the surface of the core.A novel catalyst composition is provided comprising an inner core portion and an outer portion disposed as a porous shell around the inner portion, wherein the inner portion consists essentially of metallosilicate zeolite having a medium pore structure, such as ZSM-5 or ZSM-23, and the outer portion comprising a fluoride-containing crystalline shell consisting essentially of silica substantially free of acid sites and having substantially the same crystalline structure as the inner core portion.

    Abstract translation: 通过在中孔金属硅酸盐芯上通过使二氧化硅结晶形成二氧化硅壳来制备可用于将低分子量烯烃转化为液体烃如汽油，馏出物和高粘度润滑油的表面活性形状选择性金属硅酸盐催化剂 氟离子存在于芯的表面上。 提供了一种新颖的催化剂组合物，其包括内芯部分和围绕内部部分设置为多孔壳体的外部部分，其中内部部分基本上由具有中孔结构的金属硅酸盐沸石如ZSM-5或ZSM-23组成， 并且外部部分包含基本上由基本上不含酸性部位的二氧化硅组成并且具有与内芯部分基本相同的晶体结构的含氟化物结晶壳。

    High equilibrium activity additive catalyst for catalytic cracking
    40.
    发明授权
    High equilibrium activity additive catalyst for catalytic cracking 失效
    用于催化裂化的高平衡活性添加剂催化剂

    公开(公告)号：US4818738A

    公开(公告)日：1989-04-04

    申请号：US130491

    申请日：1987-12-09

    Applicant: Pochen Chu ,  Sadi Mizrahi

    Inventor： Pochen Chu ,  Sadi Mizrahi

    IPC: B01J29/40 ,  C10G11/05 ,  B01J29/04 ,  B01J29/06

    CPC classification number: B01J29/40 ,  C10G11/05 ,  B01J2229/26 ,  B01J2229/36 ,  B01J2229/42

    Abstract: Octane and improvement in catalytic cracking processes can be attained by the addition to conventional cracking catalysts of small amounts of additive catalyst comprising a class of zeolites characterized by a silica to alumina mole ratio greater than about 12 and a Constraint Index of about 1 to 12 bound in a matrix chosen such that the matrix component forms a thermodynamically favored compound with selected cations. Sustained catalytic activity is achieved by pre-exchanging the catalyst to a high level of selected cation loading. By extending the active life of the additive catalyst, markedly lower makeup catalyst addition rates are required.

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