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公开(公告)号：US20100111796A1
公开(公告)日：2010-05-06
申请号：US12263871
申请日：2008-11-03
CPC分类号： B01D53/9468 , B01D53/9418 , B01D53/9436 , B01D2251/2062 , B01D2255/102 , B01D2255/104 , B01D2255/106 , B01D2255/20738 , B01D2255/20761 , B01D2255/50 , B01D2258/012 , B01J23/42 , B01J29/72 , B01J29/7615 , B01J35/0006 , B01J35/04 , B01J37/0225 , B01J37/0244 , B01J37/0246 , Y02A50/2325 , Y02C20/10 , Y02T10/24 , Y10T428/24149
摘要： Catalysts, methods of preparing catalyst, and methods for treating exhaust gas streams are described. In one or more embodiments, a catalyst system includes an upstream zone effective to catalyze the conversion of a mixture of NOx and NH3 to N2, and a downstream zone effective for the conversion of ammonia to N2 in the presence or absence of NOx. In an embodiment, a method for preparing a catalyst system includes: first coating one end of a substrate along at least 5% of its length with an undercoat washcoat layer containing a material composition effective to catalyze the removal of ammonia; second coating with an overcoat layer containing a material composition effective to catalyze the conversion of a mixture of NOx and NH3 to N2. A method for treating the exhaust gas stream is provided, which includes injecting ammonia or an ammonia precursor into an exhaust gas stream of a vehicle, passing the engine exhaust gas stream containing NOx and NH3 through the upstream zone of a catalyst system to remove NOx and then passing the exhaust gas stream through the downstream zone of the catalyst system to remove NH3, as well as other oxidizable species such as hydrocarbons and CO.
摘要翻译： 描述了催化剂，制备催化剂的方法和处理废气流的方法。 在一个或多个实施方案中，催化剂体系包括有效催化NOx和NH 3的混合物转化为N 2的上游区，以及在存在或不存在NO x的情况下有效地将氨转化为N 2的下游区。 在一个实施方案中，制备催化剂体系的方法包括：首先用至少5％长度的基材的一端涂覆含有有效催化去除氨的材料组合物的底涂层涂层; 第二次涂覆，其中包含有效催化NOx和NH 3的混合物转化为N 2的材料组合物的外涂层。 提供了一种处理废气流的方法，其包括将氨或氨前体注入车辆的废气流中，使含有NOx和NH 3的发动机废气流通过催化剂系统的上游区以除去NOx和 然后使废气流通过催化剂体系的下游区以除去NH 3，以及其它可氧化物质如烃和CO。
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42.发明申请公开(公告)号：US20070299278A1
公开(公告)日：2007-12-27
申请号：US11767782
申请日：2007-06-25
申请人： Claus HECHLER , Wilhelm Ruppel , Gotz-Peter Schindler , Catharina Klanner , Hans-Jurgen Bassler , Martin Dieterle , Karl-Heinrich Klappert , Klaus Joachim Muller-Engel
发明人： Claus HECHLER , Wilhelm Ruppel , Gotz-Peter Schindler , Catharina Klanner , Hans-Jurgen Bassler , Martin Dieterle , Karl-Heinrich Klappert , Klaus Joachim Muller-Engel
IPC分类号： C07C5/327 , C07C67/317 , C07C5/373
CPC分类号： C07C5/333 , B01J8/067 , B01J19/02 , B01J2219/0236 , C07C51/215 , C22C30/00 , C22C38/40 , Y02P20/52 , C07C11/06 , C07C11/02 , C07C57/04
摘要： A process for continuous heterogeneously catalyzed partial dehydrogenation of at least one hydrocarbon to be dehydrogenated in a reactor which is manufactured from a composite material which consists, on its side in contact with the reaction chamber, of a steel B with specific elemental composition which, on its side facing away from the reaction chamber, either directly or via an intermediate layer of copper, or of nickel, or of copper and nickel, is plated onto a steel A with specific elemental composition, and also partial oxidations of the dehydrogenated hydrocarbon and the reactor itself.
摘要翻译： 在反应器中连续不均匀催化的待脱氢烃的部分脱氢的方法，该反应器由复合材料制成，该复合材料在其与反应室接触的一侧由具有特定元素组成的钢B组成， 其直接或经由铜或镍或铜和镍的中间层离开反应室的一侧被镀在具有特定元素组成的钢A上，并且还将脱氢烃和 反应堆本身。
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43.发明申请公开(公告)号：US20070123732A1
公开(公告)日：2007-05-31
申请号：US11555474
申请日：2006-11-01
CPC分类号： C07C45/35 , B01J8/0469 , B01J2208/00274 , B01J2208/00495 , C07C45/33 , C07C51/215 , C07C51/252 , C07C47/22 , C07C57/04
摘要： A process for stably operating a continuous preparation process for obtaining acrolein or acrylic acid or a mixture thereof from propane, in which the feed rate of fresh propane to the process is utilized as a correcting element for stable steady-state operation.
摘要翻译： 用于稳定操作从丙烷得到丙烯醛或丙烯酸或其混合物的连续制备方法，其中将新鲜丙烷进料至该方法的进料速率用作稳定稳态操作的校正元件。
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44.发明申请PROCESS FOR PREPARING ACROLEIN OR ACRYLIC ACID OR A MIXTURE THEREOF FROM PROPANE 有权制备丙烯酸或丙烯酸或其混合物的方法公开(公告)号：US20070088092A1
公开(公告)日：2007-04-19
申请号：US11533177
申请日：2006-09-19
申请人： Catharina Klanner , Martin Dieterle , Gotz-Peter Schindler , Tsung-Chieh Cheng , Klaus Muller-Engel
发明人： Catharina Klanner , Martin Dieterle , Gotz-Peter Schindler , Tsung-Chieh Cheng , Klaus Muller-Engel
IPC分类号： C07B63/02
CPC分类号： B01J8/067 , B01J8/0415 , B01J2208/00814 , B01J2208/00849 , B01J2208/025 , C07C45/33 , C07C45/35 , C07C51/215 , C07C51/252 , C07C47/22 , C07C57/04
摘要： A process for preparing acrolein or acrylic acid or a mixture thereof from propane, in which propane is dehydrogenated under heterogeneous catalysis in a reaction zone A and the propylene formed is partially oxidized heterogeneously in a reaction zone, reaction zone A being operated in loop mode and reaction gas mixture input stream A fed to the reaction zone A comprising added molecular hydrogen which is added to this input stream as late as possible.
摘要翻译： 由丙烷制备丙烯醛或丙烯酸或其混合物的方法，其中丙烷在反应区A中在非均相催化下脱氢，形成的丙烯在反应区中部分氧化，反应区A以循环模式操作， 反应气体混合物输入流A，其进料到反应区A，其包含加入的分子氢，其尽可能晚地加入到该输入流中。
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45.发明申请Process for preparing at least one target product by partial oxidation and/or ammoxidation of propylene 有权通过丙烯的部分氧化和/或氨氧化制备至少一种目标产物的方法公开(公告)号：US20060258529A1
公开(公告)日：2006-11-16
申请号：US11411882
申请日：2006-04-27
IPC分类号： B01J23/00
CPC分类号： C07C51/43 , B01J23/002 , B01J23/8876 , B01J23/8885 , B01J35/0006 , B01J2523/00 , C07C45/33 , C07C45/35 , C07C51/25 , C07C51/252 , C07C253/26 , Y02P20/52 , C07C47/22 , C07C57/04 , B01J2523/17 , B01J2523/55 , B01J2523/68 , B01J2523/69 , C07C255/08 , B01J2523/36
摘要： A process for preparing at least one target product by partial oxidation and/or ammoxidation of propylene, in which the propylene source used is a propane dehydrogenation, the propane used therein being obtained by a rectificative prepurification of crude propane.
摘要翻译： 通过丙烯的部分氧化和/或氨氧化制备至少一种目标产物的方法，其中使用的丙烯源是丙烷脱氢，其中使用的丙烷是通过粗丙烷的精馏预纯化获得的。
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46.发明授权Heterogeneously catalyzed gas-phase partial oxidation of at least one organic compound 有权至少一种有机化合物的异相催化气相部分氧化公开(公告)号：US07115776B2
公开(公告)日：2006-10-03
申请号：US10460153
申请日：2003-06-13
IPC分类号： C07C51/16
CPC分类号： C07C51/252 , B01J8/003 , B01J8/008 , B01J8/067 , B01J23/002 , B01J2208/00707 , B01J2208/00752 , B01J2208/00761 , B01J2523/00 , C07C51/215 , C07C57/04 , B01J2523/12 , B01J2523/13
摘要： A process for the heterogeneously catalyzed gas-phase partial oxidation of an organic compound over a fixed catalyst bed present in a fixed-bed reactor having a plurality of catalyst tubes, in which the reduction of the quality of the catalyst load with increasing duration of operation is restored by a partial catalyst change, is described.
摘要翻译： 存在于具有多个催化剂管的固定床反应器中的固定催化剂床上的有机化合物的非均相催化气相部分氧化的方法，其中随着操作持续时间的延长，催化剂负载的质量降低 被部分催化剂改变所恢复。
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公开(公告)号：US20060199977A1
公开(公告)日：2006-09-07
申请号：US11357975
申请日：2006-02-22
IPC分类号： C07C51/42
摘要： A process for removing methacrolein from liquid phase P comprising acrylic acid as a main constituent and target product, and methacrolein as a secondary component in which the removal is effected by crystallization, the acrylic acid accumulating in the crystals formed and the methacrolein in the remaining mother liquor.
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48.发明申请Process for removing methacrylic acid from liquid phase comprising acrylic acid as a main constituent and target product, and methacrylic acid as a secondary component 有权从包含丙烯酸作为主要成分和目标产物的液相中除去甲基丙烯酸的方法和甲基丙烯酸作为次要组分公开(公告)号：US20060199976A1
公开(公告)日：2006-09-07
申请号：US11354101
申请日：2006-02-15
IPC分类号： C07C51/42
摘要： A process for removing methacrylic acid from liquid phase P comprising acrylic acid as a main constituent and target product, and methacrylic acid as a secondary component in which the removal is effected by crystallization, the acrylic acid accumulating in the crystals formed and the methacrylic acid in the remaining mother liquor.
摘要翻译： 从包含丙烯酸作为主要成分和目标产物的液相P中除去甲基丙烯酸的方法，以及甲基丙烯酸作为其中通过结晶进行除去的次要组分，在形成的晶体中积聚的丙烯酸和形成的晶体中的甲基丙烯酸 剩下的母酒。
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公开(公告)号：US20060177370A1
公开(公告)日：2006-08-10
申请号：US10567029
申请日：2004-07-30
IPC分类号： C01B19/00
CPC分类号： B01J19/2415 , B01J19/0046 , B01J19/10 , B01J19/18 , B01J23/002 , B01J27/0576 , B01J2219/00033 , B01J2219/0004 , B01J2219/00126 , B01J2219/00128 , B01J2219/00286 , B01J2219/00353 , B01J2219/00391 , B01J2219/00479 , B01J2219/00486 , B01J2219/00495 , B01J2219/0059 , B01J2219/00599 , B01J2219/00689 , B01J2219/00707 , B01J2219/00745 , B01J2219/00747 , B01J2523/00 , C40B30/08 , C40B40/18 , C40B50/08 , C40B60/14 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68
摘要： The sequential production of a library of N different solids, in particular heterogeneous catalysts, where N within a day is an integer of at least 2, is performed by a) producing at least two different sprayable solutions, emulsions and/or dispersions of elements and/or element compounds of the chemical elements present in the catalyst and optionally of dispersions of inorganic support materials, b) continuously metering the at least two different solutions, emulsions and/or dispersions in a predefined ratio into a mixing apparatus in which the solutions, emulsions and/or dispersions are homogeneously mixed, c) continuously drying the mixture removed from the mixing apparatus and recovering the dried mixture, d) changing the ratios in step b) and repeating steps b), c) and d) (N-1) times until N different dried mixtures are obtained, e) optionally shaping and optionally calcining the mixtures to give the solids.
摘要翻译： 通过a）产生N种不同固体，特别是非均相催化剂的文库，其中N在一天内是至少2的整数，其通过a）产生至少两种不同的可喷雾溶液，元素的乳液和/或分散体，以及 存在于催化剂中的化学元素的元素化合物和任选的无机载体材料的分散体，b）将预定比例的至少两种不同溶液，乳液和/或分散体连续计量成混合设备，其中溶液， 乳液和/或分散体均匀混合，c）连续干燥从混合装置中除去的混合物并回收干燥的混合物，d）改变步骤b）中的比例并重复步骤b），c）和d）（N-1 ），直到获得N种不同的干燥混合物，e）任选地成型和任选地煅烧混合物以得到固体。
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公开(公告)号：US07038082B2
公开(公告)日：2006-05-02
申请号：US10647335
申请日：2003-08-26
IPC分类号： B01J29/06
CPC分类号： C07C51/215 , B01J23/002 , B01J23/31 , B01J23/6525 , B01J23/8877 , B01J27/0576 , B01J35/002 , B01J37/0045 , B01J37/0223 , B01J2523/00 , C07C57/04 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68 , B01J2523/824 , B01J2523/845 , B01J2523/54 , B01J2523/44 , B01J2523/17 , B01J2523/847
摘要： A process for preparing a multimetal oxide material which contains the elements Mo, V and Te and/or Sb and at least one of the elements Nb, Ti, W, Ta and Ce and if desired promoters and has a specific X-ray diffraction pattern, in which process the last process step comprises washing with acidic liquids. In addition, a multimetal oxide material obtainable in such a way is used as a catalyst for heterogeneously catalyzed gas-phase partial oxidations and/or ammoxidation of hydrocarbons.
摘要翻译： 一种制备包含元素Mo，V和Te和/或Sb以及元素Nb，Ti，W，Ta和Ce中的至少一种的多金属氧化物材料的方法，并且如果需要的话，具有特定的X射线衍射图 ，其中最后的工艺步骤包括用酸性液体洗涤。 此外，可以以这种方式获得的多金属氧化物材料用作烃的非均相催化气相部分氧化和/或氨氧化的催化剂。
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