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11.发明申请公开(公告)号：US20120063978A1
公开(公告)日：2012-03-15
申请号：US13228734
申请日：2011-09-09
Applicant: Lisa S. Baugh , Pavel Kortunov , David C. Calabro , Michael Siskin
Inventor： Lisa S. Baugh , Pavel Kortunov , David C. Calabro , Michael Siskin
IPC: B01D53/62
CPC classification number: B01D53/1493 , B01D53/1475 , B01D53/62 , B01D2252/20415 , B01D2252/20421 , B01D2252/20426 , B01D2252/20431 , B01D2252/20478 , B01D2252/2056 , B01D2252/30 , Y02A50/2342 , Y02C10/04 , Y02C10/06
Abstract: Ionic liquids are capable of acting as solvents for amine CO2 absorbent compounds in CO2 separation processes and when so used enhance the sorption of the CO2 by the amine. A cyclic sorption process for separating CO2 from a gas stream, such as flue gas or natural gas, brings the gas stream into contact with an absorbent solution of an amine CO2 sorbent in an ionic liquid solvent followed by desorbing the CO2 to regenerate the amine.
Abstract translation: 离子液体能够作为二氧化碳分离过程中胺二氧化碳吸收剂化合物的溶剂，当这样使用时，胺可以增强二氧化碳的吸附。 用于从气流（例如废气或天然气）中分离CO 2的循环吸附方法使气流与胺CO 2吸附剂在离子液体溶剂中的吸收剂溶液接触，然后解吸CO 2以再生胺。
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12.发明授权
公开(公告)号：US5110572A
公开(公告)日：1992-05-05
申请号：US720105
申请日：1991-06-24
Applicant: David C. Calabro , Kirk D. Schmitt , James C. Vartuli
Inventor： David C. Calabro , Kirk D. Schmitt , James C. Vartuli
IPC: B01D53/86 , B01J20/02 , B01J29/03 , B01J29/04 , B01J29/40 , B01J29/70 , B01J29/82 , B01J29/83 , B01J29/85 , C01B37/00 , C01B37/02 , C01B37/08 , C01B39/00 , C10G11/05 , C10G47/16
CPC classification number: C10G47/16 , B01D53/8628 , B01J20/041 , B01J20/06 , B01J20/08 , B01J20/103 , B01J20/12 , B01J20/16 , B01J20/18 , B01J29/0308 , B01J29/04 , B01J29/041 , B01J29/40 , B01J29/70 , B01J29/82 , B01J29/83 , B01J29/85 , C01B37/00 , C01B37/02 , C01B37/08 , C01B39/00 , C10G11/05 , B01J2229/26 , B01J2229/32 , B01J2229/34 , B01J2229/36 , B01J2229/40 , B01J2229/42 , Y10S423/30
Abstract: This invention relates to a method for synthesizing ultra-large pore crystalline material which can be used as a sorbent or catalyst component for conversion of organic and inorganic compounds. A dialkoxyaluminoxytrialkoxysilane is added to the reaction mixture as a metal oxide source.
Abstract translation: 本发明涉及一种合成超大孔结晶材料的方法，该方法可用作转化有机和无机化合物的吸附剂或催化剂组分。 将二烷氧基氧基三烷氧基硅烷作为金属氧化物源加入到反应混合物中。
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13.发明授权公开(公告)号：US09610533B2
公开(公告)日：2017-04-04
申请号：US14791772
申请日：2015-07-06
Applicant: Dennis G. Peiffer , David C. Calabro , Quanchang Li , Mobae Afeworki , Stephen M. Cundy
Inventor： Dennis G. Peiffer , David C. Calabro , Quanchang Li , Mobae Afeworki , Stephen M. Cundy
IPC: C07C211/13 , C07C211/14 , C08J9/00 , B01J20/26 , B01J20/28 , B01J20/30 , C08G73/00 , C08G73/02 , B01D53/02 , B01D53/62 , C08J9/26 , C08J9/28 , B01J20/34 , B01D53/40 , C07C211/53 , C08J9/14
CPC classification number: B01D53/02 , B01D53/40 , B01D53/62 , B01D2251/80 , B01D2253/202 , B01D2253/311 , B01D2256/24 , B01D2257/504 , B01D2258/0283 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J20/3085 , B01J20/3425 , B01J20/3483 , B01J20/3491 , B01J2220/56 , C07C211/53 , C08G73/00 , C08G73/02 , C08G73/0206 , C08J9/141 , C08J9/26 , C08J9/28 , C08J2201/026 , C08J2201/0502 , C08J2203/14 , C08J2379/02 , Y02C10/04 , Y02C10/08 , Y02P20/152 , Y10T428/2982
Abstract: An adsorption-desorption material, in particular, crosslinked organo-amine polymeric materials having a weight average molecular weight of from about 500 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material, and linear organo-amine polymeric materials having a weight average molecular weight of from about 160 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material. This disclosure also relates in part to processes for preparing the crosslinked organo-amine materials and linear organo-amine materials. This disclosure further relates in part to the selective removal of CO2 and/or other acid gases from a gaseous stream containing one or more of these gases using the adsorption-desorption materials.
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14.发明申请公开(公告)号：US20150306535A1
公开(公告)日：2015-10-29
申请号：US14791833
申请日：2015-07-06
Applicant: Dennis G. Peiffer, JR. , David C. Calabro , Li Quanchang , Stephen M. Cundy
Inventor： Dennis G. Peiffer, JR. , David C. Calabro , Li Quanchang , Stephen M. Cundy
CPC classification number: B01D53/02 , B01D53/40 , B01D53/62 , B01D2251/80 , B01D2253/202 , B01D2253/311 , B01D2256/24 , B01D2257/504 , B01D2258/0283 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J20/3085 , B01J20/3425 , B01J20/3483 , B01J20/3491 , B01J2220/56 , C07C211/53 , C08G73/00 , C08G73/02 , C08G73/0206 , C08J9/141 , C08J9/26 , C08J9/28 , C08J2201/026 , C08J2201/0502 , C08J2203/14 , C08J2379/02 , Y02C10/04 , Y02C10/08 , Y02P20/152 , Y10T428/2982
Abstract: An adsorption-desorption material, in particular, crosslinked organo-amine polymeric materials having a weight average molecular weight of from about 500 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material, and linear organo-amine polymeric materials having a weight average molecular weight of from about 160 to about 1×106, a total pore volume of from about 0.2 cubic centimeters per gram (cc/g) to about 2.0 cc/g, and an adsorption capacity of at least about 0.2 millimoles of CO2 adsorbed per gram of adsorption-desorption material. This disclosure also relates in part to processes for preparing the crosslinked organo-amine materials and linear organo-amine materials. This disclosure further relates in part to the selective removal of CO2 and/or other acid gases from a gaseous stream containing one or more of these gases using the adsorption-desorption materials.
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公开(公告)号：US20140186246A1
公开(公告)日：2014-07-03
申请号：US14089055
申请日：2013-11-25
Applicant: David C. Calabro , Quanchang Li , Dennis G. Peiffer , Mobae Afeworki , Stephen M. Cundy , Charanjit S. Paur , Peter I. Ravikovitch
Inventor： David C. Calabro , Quanchang Li , Dennis G. Peiffer , Mobae Afeworki , Stephen M. Cundy , Charanjit S. Paur , Peter I. Ravikovitch
CPC classification number: B01J20/3085 , B01D53/02 , B01D53/62 , B01D2253/202 , B01D2257/504 , B01J20/262 , B01J20/264 , B01J20/267 , B01J20/3064 , B01J20/3078 , C08G77/26 , C08L83/08 , Y02C10/04 , Y02C10/06 , Y02C10/08 , Y02P20/152
Abstract: Methods are provided for synthesizing novel types of self-assembled siloxanes, such as polysiloxanes, with a sufficiently high density of amine functional groups to be useful for CO2 capture and release processes. Additionally, it has been unexpectedly found that some self-assembled polysiloxanes can be used for high temperature adsorption of CO2.
Abstract translation: 提供了用于合成新类型的自组装硅氧烷（例如聚硅氧烷）的方法，其具有足够高密度的胺官能团以用于CO 2捕获和释放过程。 另外，意外地发现一些自组装聚硅氧烷可用于高温吸附二氧化碳。
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Patent Agency Ranking
公开(公告)号：US20140178278A1
公开(公告)日：2014-06-26
申请号：US14087377
申请日：2013-11-22
Applicant: Michael Siskin , Patrick L. Hanks , Pavel Kortunov , Robert B. Fedich , Patrick P. McCall , Hans Thomann , Daniel Leta , Lisa S. Baugh , David C. Calabro , Harry W. Deckman
Inventor： Michael Siskin , Patrick L. Hanks , Pavel Kortunov , Robert B. Fedich , Patrick P. McCall , Hans Thomann , Daniel Leta , Lisa S. Baugh , David C. Calabro , Harry W. Deckman
IPC: B01D53/62
CPC classification number: B01D53/62 , B01D53/1425 , B01D53/1475 , B01D2252/20415 , B01D2252/20447 , B01D2252/20484 , Y02A50/2342 , Y02C10/04 , Y02C10/06
Abstract: Systems and methods are provided for performing CO2 sorption and regeneration processes that can take advantage of phase changes between solutions of amine-CO2 reaction products and precipitate slurries, where the slurry particles can include solid precipitates formed based on the amine-CO2 reaction products. An amine solution can be used to capture CO2 from a gas phase stream. During this initial capture process, the amine-CO2 reaction product can remain in solution. The solution containing the amine-CO2 reaction product can then be exposed to a set of conditions which result in precipitation of a portion of the amine-CO2 reaction product to form a slurry. The precipitate slurry can be passed into one or more release stages where the conditions for the slurry are altered to allow for release of the CO2.
Abstract translation: 提供了系统和方法，用于执行CO2吸附和再生过程，可以利用胺-CO 2反应产物和沉淀物浆料的溶液之间的相变，其中浆料颗粒可以包括基于胺-CO 2反应产物形成的固体沉淀物。 胺溶液可用于从气相物流中捕获CO 2。 在该初始捕获过程中，胺-CO 2反应产物可以保留在溶液中。 然后可以将含有胺-CO 2反应产物的溶液暴露于导致部分胺-CO 2反应产物沉淀形成浆料的一组条件。 沉淀浆料可以进入一个或多个释放阶段，其中改变浆料的条件以允许CO 2的释放。
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17.发明申请Polyvinyl-Amine Acid Gas Adsorption-Desorption Polymers, Processes for Preparing Same, and Uses Thereof 有权聚乙烯基胺酸气体吸附 - 解吸聚合物，其制备方法及其用途公开(公告)号：US20120164045A1
公开(公告)日：2012-06-28
申请号：US13332560
申请日：2011-12-21
Applicant: Dennis G. Peiffer , David C. Calabro , Quanchang Li , Mobae Afeworki
Inventor： Dennis G. Peiffer , David C. Calabro , Quanchang Li , Mobae Afeworki
IPC: B01D53/02 , B01D53/047 , C08J9/228 , C08G61/12
CPC classification number: C08J9/28 , B01D53/02 , B01D53/0462 , B01D53/047 , B01D53/62 , B01D2253/202 , B01D2253/311 , B01D2257/304 , B01D2257/504 , C08J9/26 , C08J2201/026 , C08J2201/0502 , C08J2339/02 , Y02C10/04 , Y02C10/08 , Y02P20/152
Abstract: This disclosure involves an adsorption-desorption material, e.g., crosslinked polyvinyl-amine material having an Mw from about 500 to about 1×106, total pore volume from about 0.2 cc/g to about 2.0 cc/g, and a CO2 adsorption capacity of at least about 0.2 millimoles per gram of crosslinked material, and/or linear polyvinyl-amine material having an Mw from about 160 to about 1×106, total pore volume from about 0.2 cc/g to about 2.0 cc/g, and a CO2 adsorption capacity of at least about 0.2 millimoles per gram of linear material. This disclosure also involves processes for preparing the crosslinked polyvinyl-amine materials and linear polyvinyl-amine materials, as well as selective removal of CO2 and/or other acid gases from a gaseous stream using the polyvinyl-amine materials.
Abstract translation: 该公开内容涉及吸附 - 解吸材料，例如具有约500至约1×10 6的Mw，约0.2cc / g至约2.0cc / g的总孔体积的交联聚乙烯胺材料和CO 2吸附容量 至少约0.2毫摩尔/克交联材料，和/或Mw为约160至约1×10 6，总孔体积为约0.2cc / g至约2.0cc / g的直链聚乙烯胺材料，以及CO 2 至少约0.2毫摩尔每克线性材料的吸附容量。 本公开还涉及制备交联聚乙烯胺材料和线性聚乙烯胺材料的方法，以及使用聚乙烯基胺材料从气流中选择性除去CO 2和/或其它酸性气体。
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公开(公告)号：US20120063979A1
公开(公告)日：2012-03-15
申请号：US13228999
申请日：2011-09-09
Applicant: Pavel Kortunov , Lisa S. Baugh , David C. Calabro , Michael Siskin
Inventor： Pavel Kortunov , Lisa S. Baugh , David C. Calabro , Michael Siskin
IPC: B01D53/62
CPC classification number: B01D53/1493 , B01D53/1475 , B01D53/62 , B01D2252/20415 , B01D2252/20421 , B01D2252/20426 , B01D2252/20431 , B01D2252/20478 , B01D2252/2056 , B01D2252/30 , Y02A50/2342 , Y02C10/04 , Y02C10/06
Abstract: A CO2 amine scrubbing process uses an absorbent mixture combination of an amine containing a primary amino group CO2 sorbent in combination with a non-nucleophilic relatively stronger base. The weaker base(s) are nucleophilic and have the ability to react directly with the CO2 in the gas stream while the relatively stronger bases act as non-nucleophilic promoters for the reaction between the CO2 and the weaker base. Two moles of CO2 can be taken up by the primary amine groups in a dicarboxylation reaction, affording the potential for a highly efficient scrubbing process.
Abstract translation: CO 2胺洗涤方法使用含有伯氨基CO 2吸附剂的胺与非亲核相对较强的碱的组合的吸收混合物组合。 较弱的碱是亲核的，并且具有与气流中的CO 2直接反应的能力，而相对较强的碱作为CO 2和较弱碱之间的反应的非亲核促进剂。 在二羧酸化反应中，二元醇可以被伯胺基团吸收，提供高效洗涤过程的潜力。
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公开(公告)号：US20120061614A1
公开(公告)日：2012-03-15
申请号：US13228652
申请日：2011-09-09
Applicant: David C. Calabro , Lisa S. Baugh , Pavel Kortunov , Benjamin A. McCool , Michael Siskin , Dennis G. Peiffer , Quanchang Li
Inventor： David C. Calabro , Lisa S. Baugh , Pavel Kortunov , Benjamin A. McCool , Michael Siskin , Dennis G. Peiffer , Quanchang Li
CPC classification number: B01D53/1493 , B01D53/1475 , B01D53/62 , B01D2252/20415 , B01D2252/20421 , B01D2252/20426 , B01D2252/20431 , B01D2252/20478 , B01D2252/2056 , B01D2252/30 , Y02A50/2342 , Y02C10/04 , Y02C10/06
Abstract: A method is described for separating CO2 and/or H2S from a mixed gas stream by contacting the gas stream with a non-aqueous, liquid absorbent medium of a primary and/or secondary aliphatic amine, preferably in a non-aqueous, polar, aprotic solvent under conditions sufficient for sorption of at least some of the CO2. The solution containing the absorbed CO2 can then be treated to desorb the acid gas. The method is usually operated as a continuous cyclic sorption-desorption process, with the sorption being carried out in a sorption zone where a circulating stream of the liquid absorbent contacts the gas stream to form a CO2-rich sorbed solution, which is then cycled to a regeneration zone for desorption of the CO2 (advantageously at 0.5:1 (approaching 1:1) may be achieved.
Abstract translation: 描述了一种从混合气流中分离CO 2和/或H 2 S的方法，其通过使气流与初级和/或仲脂族胺的非水性液体吸收介质接触，优选非水性，极性，非质子 溶剂在足以吸附至少一些CO 2的条件下进行。 然后可以处理含有吸收的CO 2的溶液以解吸酸性气体。 该方法通常作为连续循环吸附 - 脱附方法运行，吸附在吸附区中进行，其中液体吸收剂的循环流与气体流接触以形成富含CO 2的吸附剂溶液，然后循环至 用于解吸CO 2的再生区（有利地<100℃）。 在释放CO 2时，再生的贫溶液可以再循环到吸附塔。 CO 2：（初级+仲胺）吸附摩尔比> 0.5:1（接近1：1）。
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公开(公告)号：US20110150730A1
公开(公告)日：2011-06-23
申请号：US12973562
申请日：2010-12-20
Applicant: Lisa S. Baugh , David C. Calabro , Quanchang Li , Enock Berluche
Inventor： Lisa S. Baugh , David C. Calabro , Quanchang Li , Enock Berluche
CPC classification number: B01J20/2805 , B01D53/1475 , B01D53/1493 , B01D2252/20415 , B01D2252/20421 , B01D2252/20426 , B01D2252/20431 , B01D2252/20436 , B01D2258/0283 , B01J20/103 , B01J20/265 , B01J20/2803 , B01J20/28057 , B01J20/28083 , B01J20/28097 , B01J20/3204 , B01J20/3272 , C08G73/0206 , C08G73/0213 , Y02C10/04 , Y02C10/06 , Y02C10/08 , Y02P20/152
Abstract: Improved CO2 sorbents comprised of a mesoporous silica functionalized with a polyamine are obtained by the in-situ polymerization of azetidine. Also included herein are processes utilizing the improved CO2 sorbents wherein CO2 is chemisorbed onto the polyamine portion of the sorbent and the process is thermally reversible.
Abstract translation: 通过氮杂环丁烷的原位聚合获得由多胺官能化的介孔二氧化硅组成的改进的二氧化碳吸附剂。 本文还包括利用改进的CO 2吸附剂的方法，其中CO 2被化学吸附到吸附剂的多胺部分上，并且该方法是热可逆的。
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