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    Metals tolerant catalytic cracking catalyst, method of manufacture and use thereof
    24.
    发明授权
    Metals tolerant catalytic cracking catalyst, method of manufacture and use thereof 失效
    金属耐受催化裂化催化剂，其制造方法和用途

    公开(公告)号：US4938863A

    公开(公告)日：1990-07-03

    申请号：US206242

    申请日：1988-06-10

    申请人： Thomas F. Degnan ,  Billy K. Huh

    发明人： Thomas F. Degnan ,  Billy K. Huh

    IPC分类号： C10G11/05

    CPC分类号： C10G11/05

    摘要： A catalytic cracking catalyst and process which tolerates high levels of vanadium and coke precursors in the feed is disclosed. A zeolite in an alumina free binder or coating, preferably silica, is used as the cracking catalyst. RE-USY in silica is especially preferred as it has a low affinity for vanadium, low coking characteristics and high stability. Preferably a vanadium getter additive is present as separate particles to act as a vanadium sink. The catalyst and process may be used in fluidized bed catalytic cracking (FCC) or in moving bed catalytic cracking units. A method of making a coated catalyst, by adding a layer of an alumina free material to a core of alumina containing cracking catalyst is also disclosed.

    摘要翻译： 公开了一种催化裂化催化剂和方法，其耐受饲料中高含量的钒和焦炭前体。 使用不含氧化铝的粘合剂或涂层中的沸石，优选二氧化硅作为裂化催化剂。 二氧化硅中的RE-USY是特别优选的，因为它对钒的低亲和力，低焦化特性和高稳定性。 优选地，钒吸附剂添加剂作为单独的颗粒存在以充当钒槽。 催化剂和方法可用于流化床催化裂化（FCC）或移动床催化裂化装置。 还公开了通过向含氧化铝的裂化催化剂的核心添加无氧化铝材料层来制备涂覆的催化剂的方法。

    Manufacture of improved catalyst
    29.
    发明授权
    Manufacture of improved catalyst 失效
    改良催化剂的制造

    公开(公告)号：US5472922A

    公开(公告)日：1995-12-05

    申请号：US140936

    申请日：1993-10-25

    申请人： Thomas F. Degnan ,  Terry E. Helton ,  Grant H. Yokomizo

    发明人： Thomas F. Degnan ,  Terry E. Helton ,  Grant H. Yokomizo

    IPC分类号： B01J29/70 ,  B01J29/04

    CPC分类号： B01J29/7007 ,  B01J2229/26 ,  B01J2229/36 ,  B01J2229/42

    摘要： Methods for preparing phosphorus containing catalysts comprising a large-pore zeolite, e.g., zeolite Beta, zeolite ZSM-12, or zeolite ZSM-20, and a matrix which have improved attrition resistance. The present invention includes the catalyst compositions produced by the above methods. Also included in the present invention are methods for the use of catalysts prepared by the present method in hydrocarbon cracking processes. It is desired to develop cracking catalysts for organic compound conversion that have improved cracking yields and have good attrition resistance. This invention involves the use of large pore siliceous zeolites and a highly siliceous matrix to produce a cracking catalyst with improved cracking yields and good attrition resistance. The invention further involves the use of phosphorus and the use of selected sequences for combining the compounds in the manufacture of the catalyst to enhance the attrition resistance of the catalyst.

    摘要翻译： 制备含有大孔沸石的含磷催化剂的方法，例如β沸石沸石，沸石ZSM-12或沸石ZSM-20，以及具有改善耐磨性的基体。 本发明包括通过上述方法制备的催化剂组合物。 本发明还包括使用本方法制备的催化剂在烃裂解方法中的方法。 需要开发有机化合物转化的裂化催化剂，其具有改善的裂化产率并具有良好的耐磨性。 本发明涉及使用大孔硅质沸石和高度硅质基质来生产具有改进的裂化产率和良好耐磨性的裂化催化剂。 本发明进一步涉及磷的使用和选择的序列用于在催化剂制造中组合化合物以提高催化剂耐磨耗性的用途。

    Manufacture of improved zeolite Beta catalyst
    30.
    发明授权
    Manufacture of improved zeolite Beta catalyst 失效
    改良沸石β催化剂的制造

    公开(公告)号：US5457078A

    公开(公告)日：1995-10-10

    申请号：US158325

    申请日：1993-11-29

    申请人： Robert P. L. Absil ,  Thomas F. Degnan ,  George H. Hatzikos ,  Jocelyn A. Kowalski ,  Thomas Mebrahtu ,  Grant H. Yokomizo

    发明人： Robert P. L. Absil ,  Thomas F. Degnan ,  George H. Hatzikos ,  Jocelyn A. Kowalski ,  Thomas Mebrahtu ,  Grant H. Yokomizo

    IPC分类号： B01J29/40 ,  B01J29/70 ,  B01J37/00 ,  C10G11/05 ,  B01J29/06 ,  B01J27/14

    CPC分类号： C10G11/05 ,  B01J29/7007 ,  B01J37/0009 ,  B01J2229/26 ,  B01J2229/36 ,  B01J2229/42 ,  B01J29/40 ,  B01J29/7034 ,  B01J29/7042

    摘要： A catalyst composition which comprises a crystalline metallosilicate having the structure of zeolite Beta, phosphorus, and a matrix that is substantially free of crystalline aluminum phosphate which has improved resistance to steam deactivation and which has higher cracking activity than analogous catalysts prepared without phosphorus. The crystalline metallosilicate may be used in the as-synthesized form or in the calcined form. Also included is the method to produce the catalyst composition and methods for the use of catalysts prepared by the present method in organic conversion processes. Specific embodiments of the invention involve various techniques for preparation of catalysts containing phosphorus and crystalline metallosilicates having the structure of zeolite Beta. Catalysts prepared according to the method of this invention are useful for organic compound, e.g., hydrocarbon compound, conversion processes. Organic compound conversion processes include cracking, hydrocracking, and transalkylation, among others.

    摘要翻译： 一种催化剂组合物，其包含具有沸石β，磷的结构的结晶金属硅酸盐和基本上不含结晶磷酸铝的基质，其具有改善的对蒸汽失活的抗性，并且具有比不含磷制备的类似催化剂更高的裂化活性。 结晶金属硅酸盐可以以合成形式或以煅烧形式使用。 还包括制备催化剂组合物的方法和使用通过本发明方法制备的催化剂在有机转化方法中的方法。 本发明的具体实施方案涉及用于制备含有β沸石结构的含有磷的结晶金属硅酸盐的催化剂的各种技术。 根据本发明方法制备的催化剂可用于有机化合物，例如烃化合物，转化方法。 有机化合物转化方法包括裂化，加氢裂化和烷基转移等。