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    Methanol synthesis
    2.
    发明授权
    Methanol synthesis 失效
    甲醇合成

    公开(公告)号：US07696390B2

    公开(公告)日：2010-04-13

    申请号：US12136142

    申请日：2008-06-10

    申请人： John E. Stauffer

    发明人： John E. Stauffer

    IPC分类号： C07C29/14

    CPC分类号： C07C17/154 ,  C07C17/23 ,  C07C29/141 ,  C07C45/43 ,  C07C19/03 ,  C07C47/04 ,  C07C31/04

    摘要： A process is disclosed for the synthesis of methanol from methane comprising three reaction steps operated in tandem. In the first step methylene chloride is produced by the reaction of methane with oxygen and hydrogen chloride. In the second step, methylene chloride is hydrolyzed to formaldehyde, which is hydrogenated in the third step to provide the product methanol.

    摘要翻译： 公开了从甲烷合成甲醇的方法，其包括串联操作的三个反应步骤。 在第一步中，通过甲烷与氧气和氯化氢的反应产生二氯甲烷。 在第二步中，将二氯甲烷水解成甲醛，在第三步中氢化，得到产物甲醇。

    Process for the conversion of ethylene to vinyl chloride, and novel catalyst compositions useful for such process
    4.
    发明申请
    Process for the conversion of ethylene to vinyl chloride, and novel catalyst compositions useful for such process 审中-公开
    将乙烯转化为氯乙烯的方法和用于该方法的新型催化剂组合物

    公开(公告)号：US20050148805A1

    公开(公告)日：2005-07-07

    申请号：US11053688

    申请日：2005-02-08

    申请人： Mark Jones ,  Daniel Hickman ,  Michael Olken

    发明人： Mark Jones ,  Daniel Hickman ,  Michael Olken

    IPC分类号： B01J23/10 ,  B01J27/10 ,  B01J27/125 ,  C07C17/013 ,  C07C17/02 ,  C07C17/07 ,  C07C17/08 ,  C07C17/152 ,  C07C17/154 ,  C07C17/156 ,  C07F5/00

    CPC分类号： B01J27/125 ,  B01J23/10 ,  B01J27/10 ,  C07C17/154 ,  C07C17/156 ,  C07C21/06

    摘要： This invention is a process for producing vinyl chloride from an ethylene-containing feed, oxygen, and a chlorine source in the presence of a catalyst. The process permits direct production of vinyl chloride in a single reactor system, and further permits ethane to be used as the C2 hydrocarbon feed with recycle of ethylene from the product stream to constitute the ethylene specified for the feed. This invention in another aspect concerns also a composition of matter, and a method for making the composition, wherein the composition is useful as a catalyst for the vinyl chloride process. The composition comprises a rare earth-containing material, with the proviso that the catalyst prepared therefrom is substantially free of iron and copper and with the further proviso that when cerium is present the catalyst further comprises at least one more rare earth element other than cerium.

    摘要翻译： 本发明是在催化剂存在下由含乙烯的进料，氧气和氯源生产氯乙烯的方法。 该方法允许在单个反应器系统中直接生产氯乙烯，并且进一步允许乙烷用作C 2 O 2烃进料，其中乙烯从产物流中再循环以构成针对进料的乙烯 。 在另一方面，本发明还涉及一种物质组合物和一种制备该组合物的方法，其中该组合物可用作氯乙烯方法的催化剂。 所述组合物包含含稀土材料，条件是由其制备的催化剂基本上不含铁和铜，另外条件是当存在铈时，催化剂还包含至少一种除铈以外的至少一种稀土元素。

    Method for reducing formation of polychlorinated aromatic compounds during oxychlorination of C1-C3 hydrocarbons
    6.
    发明授权
    Method for reducing formation of polychlorinated aromatic compounds during oxychlorination of C1-C3 hydrocarbons 失效
    在C1-C3烃氧氯化期间减少多氯代芳族化合物形成的方法

    公开(公告)号：US06177599B1

    公开(公告)日：2001-01-23

    申请号：US08559123

    申请日：1995-11-17

    申请人： Joseph Allen Cowfer ,  Victor James Johnston ,  Lawrence Popiel

    发明人： Joseph Allen Cowfer ,  Victor James Johnston ,  Lawrence Popiel

    IPC分类号： C07C17154

    CPC分类号： C07C17/154 ,  C07C17/15 ,  C07C17/152 ,  C07C17/156 ,  C07C17/158

    摘要： An improved process is disclosed for manufacturing chlorinated hydrocarbon by way of oxychlorination which yields reduced levels of environmental toxins such as, chlorobenzenes, polychlorinated biphenyls, polychlorinated dibenzodioxins and polychlorinated dibenzofurans. The process involves fixed bed or fluid bed catalyzed oxychlorination of a hydrocarbon reactant containing from 1 to 3 carbon atoms. The oxychlorination process consists of contacting the hydrocarbon reactant with oxygen or oxygenated gas and at least a portion of externally obtained hydrogen chloride in the presence of the oxychlorination catalyst in a heated reaction zone operated at from 150° C. to 600° C. and recovering chlorinated hydrocarbon from the effluents of the reaction zone. The improvement consists of the use of at least a portion of the hydrogen chloride from an external source other than from recovery of hydrogen chloride from the thermal pyrolysis of the product from the operated oxychlorination process, wherein the external hydrogen chloride, containing aromatic hydrocarbons, is pretreated before use in the operated oxychlorination process by a means for removal of the aromatic hydrocarbons.

    摘要翻译： 公开了通过氧氯化生产氯化烃的改进方法，其产生环境毒素水平降低，例如氯苯，多氯联苯，多氯二苯并二恶英和多氯二苯并呋喃。 该方法涉及含有1至3个碳原子的烃反应物的固定床或流化床催化氧氯化。 氧氯化方法包括在氧化催化剂存在下，在150℃至600℃的加热反应区中使烃反应物与氧气或氧化气体和至少部分外部获得的氯化氢接触并回收 来自反应区流出物的氯化烃。 该改进包括使用来自外部来源的至少一部分氯化氢，而不是从操作的氧氯化方法从产物的热热解中回收氯化氢，其中含有芳烃的外部氯化氢是 在运行的氧氯化方法中通过除去芳族烃的方法在使用前预处理。

    Process for converting light alkanes to higher hydrocarbons
    8.
    发明授权
    Process for converting light alkanes to higher hydrocarbons 失效
    将轻质烷烃转化为高级烃的方法

    公开(公告)号：US4769504A

    公开(公告)日：1988-09-06

    申请号：US45634

    申请日：1987-03-04

    申请人： Richard P. Noceti ,  Charles E. Taylor

    发明人： Richard P. Noceti ,  Charles E. Taylor

    IPC分类号： C07C1/26 ,  C07C17/154 ,  C07C2/42

    CPC分类号： C07C1/26 ,  C07C17/154 ,  C07C2529/40 ,  Y10S585/901 ,  Y10S585/935

    摘要： A process is disclosed for the production of aromatic-rich, gasoline boiling range hydrocarbons from the lower alkanes, particularly from methane. The process is carried out in two stages. In the first, alkane is reacted with oxygen and hydrogen chloride over an oxyhydrochlorination catalyst such as copper chloride with minor proportions of potassium chloride and rare earth chloride. This produces an intermediate gaseous mixture containing water and chlorinated alkanes. The chlorinated alkanes are contacted with a crystalline aluminosilicate catalyst in the hydrogen or metal promoted form to produce gasoline range hydrocarbons with a high proportion of aromatics and a small percentage of light hydrocarbons (C.sub.2 -C.sub.4). The light hydrocarbons can be recycled for further processing over the oxyhydrochlorination catalyst.

    摘要翻译： 公开了用于从低级烷烃，特别是甲烷生产富含芳香族的汽油沸程烃的方法。 该过程分两个阶段进行。 首先，烷烃与氧氯化氢催化剂如氯化铜与少量氯化钾和稀土氯化物一起与氧和氯化氢反应。 这产生含有水和氯化烷烃的中间气体混合物。 氯化烷烃与氢或金属促进形式的结晶硅铝酸盐催化剂接触，以生产具有高比例芳族化合物和少量轻烃（C 2 -C 4）的汽油范围烃。 轻质烃可以再循环用于进一步处理氧化氢氯化催化剂。

    Process for the oxychlorination of an alkane using a solid solution catalyst containing iron cations
    10.
    发明授权
    Process for the oxychlorination of an alkane using a solid solution catalyst containing iron cations 失效
    使用含有铁阳离子的固溶体催化剂对烷烃进行氧氯化的方法

    公开(公告)号：US4375569A

    公开(公告)日：1983-03-01

    申请号：US950119

    申请日：1978-10-10

    申请人： William J. Kroenke ,  Paul P. Nicholas

    发明人： William J. Kroenke ,  Paul P. Nicholas

    IPC分类号： B01J23/745 ,  B01J23/76 ,  B01J23/86 ,  C07C17/154

    CPC分类号： B01J23/76 ,  B01J23/745 ,  B01J23/86 ,  C07C17/154

    摘要： An alkane is reacted with oxygen and available chlorine in the presence of a solid solution catalyst containing iron cations to yield unsaturated hydrocarbons and chlorinated saturated and unsaturated hydrocarbons. In a preferred embodiment of the process, ethane is reacted with oxygen and available chlorine in the presence of a solid solution catalyst containing iron cations to yield vinyl chloride, ethylene, and other valuable by-products. The conversion of ethane to products approaches 100 percent, vinyl chloride is prepared in up to 40 mole percent yield, and the combined yield of vinyl chloride, ethylene dichloride, ethyl chloride, and ethylene is up to 90 mole percent.

    摘要翻译： 在含有铁阳离子的固溶体催化剂的存在下，使烷烃与氧气和有效氯反应，得到不饱和烃和氯化饱和和不饱和烃。 在该方法的优选实施方案中，乙烷在含有铁阳离子的固溶体催化剂存在下与氧气和有效氯反应，产生氯乙烯，乙烯和其它有价值的副产物。 乙烷转化成产物接近100％，氯乙烯的制备高达40摩尔％，氯乙烯，二氯乙烷，乙基氯和乙烯的合并产率高达90％。