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    Praseodymium-palladium binary oxide, catalyst compositions containing the same, and methods of use
    41.
    发明授权
    Praseodymium-palladium binary oxide, catalyst compositions containing the same, and methods of use 失效
    镨 - 钯二元氧化物，含有其的催化剂组合物和使用方法

    公开(公告)号：US5102639A

    公开(公告)日：1992-04-07

    申请号：US684631

    申请日：1991-04-12

    申请人： Ting C. Chou ,  Teresa Kennelly ,  Robert J. Farrauto

    发明人： Ting C. Chou ,  Teresa Kennelly ,  Robert J. Farrauto

    IPC分类号： B01J23/63 ,  B01J23/96 ,  B01J38/12 ,  C01G55/00 ,  F23C13/00

    CPC分类号： B01J23/63 ,  C01G55/00 ,  Y02P20/584

    摘要： A novel praseodymium-palladium oxide compound has the formula Pr.sub.4 PdO.sub.7. The compound has utility as a catalyst for oxidation of combustion mixtures comprising oxygen (e.g., air) and gaseous carbonaceous fuels such as methane and displays excellent regeneration characteristics after exposure to decomposition-causing temperatures. The compound may be used in a catalyst composition by being coated as a washcoat on a suitable carrier. Catalytic combustion processes are carried out by contacting such combustion mixture with the catalyst under combustion conditions, including catalytically supported thermal combustion. Regeneration of over-temperatured catalyst is also provided for.

    摘要翻译： 一种新型的镨 - 氧化钯化合物具有式Pr4PdO7。 该化合物具有用于氧化包含氧（例如空气）和气态碳质燃料如甲烷的燃烧混合物的催化剂的效用，并且在暴露于分解引起的温度之后显示优异的再生特性。 该化合物可以通过在合适的载体上涂覆作为修补基面涂料而用于催化剂组合物中。 催化燃烧过程通过使燃烧混合物与催化剂在燃烧条件下接触进行，包括催化负载的热燃烧。 还提供过温催化剂的再生。

    Methods and systems for generating hydrogen and separating carbon dioxide
    44.
    发明授权
    Methods and systems for generating hydrogen and separating carbon dioxide 有权
    用于产生氢气和分离二氧化碳的方法和系统

    公开(公告)号：US08926942B2

    公开(公告)日：2015-01-06

    申请号：US12679506

    申请日：2008-02-22

    申请人： Marco J. Castaldi ,  Robert J. Farrauto ,  Tuncel M. Yegulalp

    发明人： Marco J. Castaldi ,  Robert J. Farrauto ,  Tuncel M. Yegulalp

    IPC分类号： C01B31/18 ,  B01D53/02 ,  C01B3/38 ,  C01B3/48 ,  C01B3/56

    CPC分类号： B01D53/02 ,  B01D2253/112 ,  B01D2256/16 ,  B01D2257/504 ,  B01D2259/122 ,  C01B3/38 ,  C01B3/48 ,  C01B3/56 ,  C01B2203/0233 ,  C01B2203/0283 ,  C01B2203/0425 ,  C01B2203/0475 ,  C01B2203/06 ,  C01B2203/066 ,  C01B2203/1064 ,  C01B2203/1235 ,  C01B2203/82 ,  Y02C10/08 ,  Y02P20/152

    摘要： Methods and systems for generating hydrogen and separating carbon dioxide from a feed stream including hydro-carbons and water are disclosed. In some embodiments, the method includes the following: providing a catalytic chamber including a monolithic structure having surfaces coated with carbon dioxide adsorbing materials and one or more washcoated layers of combined steam reforming, water gas shift, and combustion catalysts; directing the feed stream into said catalytic chamber; controlling the feed stream so that it has a temperature range that allows the reactive generation of carbon dioxide and hydrogen gas but does not cause substantial development of coke between hydrocarbons in the feed stream and said surfaces of said monolithic structure; and adsorbing said carbon dioxide generated by heating the feed stream, wherein said carbon dioxide is adsorbed onto carbon dioxide adsorbing materials on said surfaces of said monolithic structure.

    摘要翻译： 公开了用于产生氢气并从包括氢碳和水的进料流中分离二氧化碳的方法和系统。 在一些实施方案中，该方法包括以下：提供催化室，其包括具有涂覆有二氧化碳吸附材料的表面的整体结构和一个或多个组合的蒸汽重整，水煤气变换和燃烧催化剂的洗涂层; 将进料流引导到所述催化室中; 控制进料流，使其具有允许反应生成二氧化碳和氢气的温度范围，但不会引起进料流中的烃和所述整体式结构的所述表面之间的焦炭的显着发展; 并且通过加热所述进料流而吸收所述二氧化碳，其中所述二氧化碳被吸附在所述整体式结构的所述表面上的二氧化碳吸附材料上。

    Catalytic oxidation method
    47.
    发明授权
    Catalytic oxidation method 失效
    催化氧化法

    公开(公告)号：US06153160A

    公开(公告)日：2000-11-28

    申请号：US405279

    申请日：1995-03-16

    申请人： Kenneth E. Voss ,  Bulent O. Yavuz ,  Robert J. Farrauto ,  Michael P. Galligan

    发明人： Kenneth E. Voss ,  Bulent O. Yavuz ,  Robert J. Farrauto ,  Michael P. Galligan

    IPC分类号： B01D53/86 ,  B01D53/94 ,  B01J23/10 ,  B01J23/40 ,  B01J23/63 ,  B01J35/10 ,  B01J37/02 ,  F02B3/06 ,  F24C15/20 ,  B01J8/04

    CPC分类号： B01J37/0244 ,  B01D53/864 ,  B01D53/944 ,  B01J23/10 ,  B01J23/63 ,  B01J35/10 ,  B01J37/0215 ,  B01J35/1014 ,  B01J35/1019 ,  F02B3/06

    摘要： Oxidation catalyst compositions include a catalytic material having a BET surface area of at least about 10 m.sup.2 /g and consists of a combination of bulk ceria and a bulk second metal oxide which may be one or more of titania, zirconia, ceria-zirconia, silica, alumina-silica and .alpha.-alumina. The combination may optionally also include activated alumina having a BET surface area of at least about 10 m.sup.2 /g. The ceria, second metal oxide and optional activated alumina may be mixed together or provided as discrete layers. Optionally, one of platinum or palladium metal may be dispersed on the catalytic material provided that the platinum, when used, is used in limited amounts to preclude excessive oxidation of SO.sub.2 to SO.sub.3. The catalyst compositions may be used for oxidation of oxidizeable components in a gas-borne stream, e.g., in a method to treat diesel engine exhaust by contacting the hot exhaust with the catalyst composition to promote the oxidation of the volatile organic fraction. The optional inclusion of platinum or palladium promotes the oxidation of gas phase components, e.g., hydrocarbons and carbon monoxide.

    摘要翻译： 氧化催化剂组合物包括具有至少约10m 2 / g的BET表面积的催化材料，并且由本体二氧化铈和块状第二金属氧化物的组合组成，其可以是二氧化钛，氧化锆，二氧化铈 - 氧化锆，二氧化硅中的一种或多种 ，氧化铝 - 二氧化硅和α-氧化铝。 该组合可以任选地还包括具有至少约10m 2 / g的BET表面积的活性氧化铝。 二氧化铈，第二金属氧化物和任选的活性氧化铝可以混合在一起或作为离散层提供。 任选地，铂或钯金属中的一种可以分散在催化材料上，条件是当使用铂时，铂被限制用于排除SO2过度氧化成SO 3。 催化剂组合物可用于氧化可气化成分的气体输送流，例如通过使热排气与催化剂组合物接触以促进挥发性有机部分的氧化来处理柴油发动机排气的方法。 铂或钯的任选包含促进气相组分如碳氢化合物和一氧化碳的氧化。

    Combustion catalysts containing binary oxides and processes using the same
    48.
    发明授权
    Combustion catalysts containing binary oxides and processes using the same 失效
    含二元氧化物的燃烧催化剂及其使用方法

    公开(公告)号：US5863851A

    公开(公告)日：1999-01-26

    申请号：US800747

    申请日：1997-02-14

    申请人： Teresa Kennelly ,  Ting C. Chou ,  Robert J. Farrauto

    发明人： Teresa Kennelly ,  Ting C. Chou ,  Robert J. Farrauto

    IPC分类号： B01J23/63 ,  B01J23/96 ,  B01J38/12 ,  C01G55/00 ,  F23C13/00 ,  B01J20/34

    CPC分类号： B01J38/12 ,  B01J23/63 ,  B01J23/96

    摘要： A catalyst composition containing one or more binary oxides of palladium and rare earth metal such as Ce, La, Nd, Pr and/or Sm. The catalyst composition is used for the catalytic combustion of gaseous combustion mixtures of oxygen and carbonaceous fuels such as methane, e.g., a natural gas/air combustion mixture. Specific preferred binary oxides may be, for example, M.sub.2 O.sub.3.PdO (e.g., La.sub.2 O.sub.3.PdO) or 2M.sub.2 O.sub.3.PdO, wherein in each case M is La, Nd or Sm. A process of combusting gaseous carbonaceous fuels includes contacting a catalyst as described above under combustion conditions, e.g., 925.degree. C. to 1650.degree. C. and 1 to 20 atmospheres pressure, to carry out sustained combustion of the combustion mixture, including catalytically supported thermal combustion. Regeneration of over-temperatured M.sub.2 O.sub.3.PdO catalyst is also provided for.

    摘要翻译： 含有一种或多种钯和稀土金属如Ce，La，Nd，Pr和/或Sm的二元氧化物的催化剂组合物。 催化剂组合物用于氧气和碳质燃料如甲烷的气体燃烧混合物的催化燃烧，例如天然气/空气燃烧混合物。 特别优选的二元氧化物可以是例如M 2 O 3 PdO（例如La 2 O 3·P 10）或2M 2 O 3·P 10，其中在每种情况下M是La，Nd或Sm。 燃烧气态含碳燃料的方法包括在燃烧条件例如925℃至1650℃和1至20大气压的压力下使如上所述的催化剂接触，以进行燃烧混合物的持续燃烧，包括催化负载的热 燃烧。 还提供了过温度M2O3.PdO催化剂的再生。

    Oxidation catalyst with bulk ceria, a second bulk metal oxide, and platinum
    50.
    发明授权
    Oxidation catalyst with bulk ceria, a second bulk metal oxide, and platinum 失效
    具有本体二氧化铈，第二块体金属氧化物和铂的氧化催化剂

    公开(公告)号：US5491120A

    公开(公告)日：1996-02-13

    申请号：US247531

    申请日：1994-05-23

    申请人： Kenneth E. Voss ,  Bulent O. Yavuz ,  Robert J. Farrauto ,  Michael P. Galligan

    发明人： Kenneth E. Voss ,  Bulent O. Yavuz ,  Robert J. Farrauto ,  Michael P. Galligan

    IPC分类号： B01D53/86 ,  B01D53/94 ,  B01J23/10 ,  B01J23/40 ,  B01J23/63 ,  B01J35/10 ,  B01J37/02 ,  F02B3/06 ,  F24C15/20 ,  B01J23/42 ,  B01J21/06 ,  B01J21/04

    CPC分类号： B01J37/0244 ,  B01D53/864 ,  B01D53/944 ,  B01J23/10 ,  B01J23/63 ,  B01J35/10 ,  B01J37/0215 ,  B01J35/1014 ,  B01J35/1019 ,  F02B3/06

    摘要： Oxidation catalyst compositions include a catalytic material having a BET surface area of at least about 10 m.sup.2 /g and consisting essentially of a combination of bulk ceria and a bulk second metal oxide which may be one or more of titania, zirconia, ceria-zirconia, silica, alumina-silica and .alpha.-alumina. The combination may optionally also include activated alumina having a BET surface area of at least about 10 m.sup.2 /g. The ceria, second metal oxide and optional activated alumina may be mixed together or provided as discrete layers. Optionally, one of platinum or palladium metal may be dispersed on the catalytic material provided that the platinum, when used, is used in limited amounts to preclude excessive oxidation of SO.sub.2 to SO.sub.3. The catalyst compositions may be used for oxidation of oxidizeable components in a gas-borne stream, e.g., in a method to treat diesel engine exhaust by contacting the hot exhaust with the catalyst composition to promote the oxidation of the volatile organic fraction. The optional inclusion of platinum or palladium promotes the oxidation of gas phase components, e.g., hydrocarbons and carbon monoxide.

    摘要翻译： 氧化催化剂组合物包括具有至少约10m 2 / g的BET表面积并且基本上由本体二氧化铈和体积第二金属氧化物的组合组成的催化材料，其可以是二氧化钛，氧化锆，二氧化铈 - 氧化锆中的一种或多种， 二氧化硅，氧化铝 - 二氧化硅和α-氧化铝。 该组合可以任选地还包括具有至少约10m 2 / g的BET表面积的活性氧化铝。 二氧化铈，第二金属氧化物和任选的活性氧化铝可以混合在一起或作为离散层提供。 任选地，铂或钯金属中的一种可以分散在催化材料上，条件是当使用铂时，铂被限制用于排除SO2过度氧化成SO 3。 催化剂组合物可用于氧化可气化成分的气体输送流，例如通过使热排气与催化剂组合物接触以促进挥发性有机部分的氧化来处理柴油发动机排气的方法。 铂或钯的任选包含促进气相组分如碳氢化合物和一氧化碳的氧化。