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    HYDROGENATED POLYMERS WITH A RADIAL STRUCTURE HAVING A CORE BASED ON CALIXARENES AND USE THEREOF IN LUBRICANT COMPOSITIONS
    5.
    发明申请
    HYDROGENATED POLYMERS WITH A RADIAL STRUCTURE HAVING A CORE BASED ON CALIXARENES AND USE THEREOF IN LUBRICANT COMPOSITIONS 审中-公开
    具有基于加仑剂的核心的径向结构的氢化聚合物及其在润滑剂组合物中的用途

    公开(公告)号：US20170051224A1

    公开(公告)日：2017-02-23

    申请号：US15304757

    申请日：2015-04-16

    申请人： ENI S.P.A. ,  Versalis S.P.A.

    发明人： Marcello NOTARI ,  Claudio CAVALLO ,  Alberto ROSELLI ,  Alessandro CASNATI ,  Francesco SANSONE ,  Alessandro BURLINI

    IPC分类号： C10M119/02 ,  C08G81/02 ,  C10M159/00

    CPC分类号： C10M119/02 ,  C08C19/02 ,  C08G81/022 ,  C10M159/005 ,  C10M2209/101 ,  C10M2213/04 ,  C10M2229/00 ,  C10N2220/029 ,  C10N2230/02 ,  C10N2230/68 ,  C10N2260/02 ,  C10N2270/00 ,  C10M2205/06 ,  C10M2205/04

    摘要： Hydrogenated polymers with a radial structure having a core made up of calixarenes of the general formula (I), to the core of which is linked a number P of hydrogenated linear polymer segments selected from: —hydrogenated homopolymers or copolymers of conjugated dienes; or —hydrogenated copolymers of said conjugated dienes and monoalkenyl arenes, and —mixtures thereof said formula (I) in which: —R1, R2, R3 and R4 are independently selected from hydrogen; a group containing carbon and hydrogen; a group also containing heteroatoms in addition to carbon and hydrogen; a group also containing silicon in addition to carbon, hydrogen and heteroatoms; —one of the two substituents R5 and R6 is hydrogen, while the other may be hydrogen or alkyl, with a number of carbon atoms between 1 and 6, preferably methyl and ethyl; —n is an integer in the range between 4 and 16.

    摘要翻译： 具有径向结构的氢化聚合物具有由通式（I）的杯芳烃构成的核心，其核心连接数个P的氢化的线性聚合物链段，其选自： ​​- 氢化均聚物或共轭二烯的共聚物; 或所述共轭二烯和单烯基芳烃的氢化共聚物，及其所述式（I）的混合物，其中：-R 1，R 2，R 3和R 4独立地选自氢; 含碳和氢的基团; 除碳和氢之外还含有杂原子的基团; 除了碳，氢和杂原子之外还含有硅的基团; 两个取代基R5和R6之一是氢，而另一个可以是氢或烷基，其中多个碳原子在1和6之间，优选甲基和乙基; - n是4和16之间的整数。

    Detergent copolymer of unsaturated polyglycol ether
    10.
    发明授权
    Detergent copolymer of unsaturated polyglycol ether 失效
    不饱和聚乙二醇醚的洗涤剂共聚物

    公开(公告)号：US3189586A

    公开(公告)日：1965-06-15

    申请号：US19783962

    申请日：1962-05-28

    申请人： CALIFORNIA RESEARCH CORP

    发明人： STUART FRANK A ,  STEWART WILLIAM T ,  WARREN LOWE ,  KAVANAGH FRANK W

    IPC分类号： C08F8/00 ,  C08F8/14 ,  C08F16/12 ,  C08F20/10 ,  C08F20/58 ,  C08F20/62 ,  C08F22/00 ,  C08F220/18 ,  C08F283/00 ,  C08F283/06 ,  C08F290/06 ,  C08L33/08 ,  C09G1/00 ,  C10M159/00

    CPC分类号： C10M159/005 ,  C08F8/00 ,  C08F16/12 ,  C08F20/58 ,  C08F20/62 ,  C08F22/00 ,  C08F220/18 ,  C08F283/00 ,  C08F283/06 ,  C08F290/062 ,  C08F2800/10 ,  C08F2800/20 ,  C10M1/08 ,  C10M3/00 ,  C10M143/00 ,  C10M143/02 ,  C10M145/02 ,  C10M147/02 ,  C10M149/02 ,  C10M151/02 ,  C10M153/02 ,  C10M2203/02 ,  C10M2203/022 ,  C10M2203/024 ,  C10M2203/04 ,  C10M2203/10 ,  C10M2205/00 ,  C10M2205/02 ,  C10M2205/022 ,  C10M2205/026 ,  C10M2205/14 ,  C10M2205/16 ,  C10M2205/17 ,  C10M2205/18 ,  C10M2205/22 ,  C10M2207/027 ,  C10M2207/282 ,  C10M2207/34 ,  C10M2209/02 ,  C10M2209/084 ,  C10M2209/103 ,  C10M2209/104 ,  C10M2209/105 ,  C10M2209/107 ,  C10M2209/108 ,  C10M2209/109 ,  C10M2213/00 ,  C10M2213/02 ,  C10M2213/04 ,  C10M2213/06 ,  C10M2215/042 ,  C10M2217/00 ,  C10M2217/02 ,  C10M2217/022 ,  C10M2217/023 ,  C10M2217/024 ,  C10M2217/026 ,  C10M2217/028 ,  C10M2217/04 ,  C10M2217/044 ,  C10M2217/045 ,  C10M2217/06 ,  C10M2219/087 ,  C10M2219/088 ,  C10M2219/089 ,  C10M2221/00 ,  C10M2221/02 ,  C10M2221/04 ,  C10M2221/041 ,  C10M2221/043 ,  C10M2223/041 ,  C10M2223/045 ,  C10M2223/12 ,  C10M2225/00 ,  C10M2225/02 ,  C10M2225/04 ,  C10M2227/02 ,  C10M2229/00 ,  C10N2210/02 ,  C10N2240/04 ,  C10N2240/042 ,  C10N2240/044 ,  C10N2240/046 ,  C10N2240/10 ,  C10N2240/101 ,  C10N2240/104 ,  C10N2240/106 ,  C10N2270/02 ,  Y10S526/933 ,  C08F8/14 ,  C08F8/12 ,  C08F120/18 ,  C08F110/10

    摘要： A lubricating composition, especially suitable for use in internal combustion engines, comprises a major proportion by weight of a lubricating oil and a minor proportion by weight, sufficient to enhance the detergent characteristics of the composition, of an additive consisting of a predominantly aliphatic or cycloaliphatic macromolecule, which macromolecule comprises up to 99,9% by weight of oil-solubilizing aliphatic or cycloaliphatic hydrocarbon groups and at least 0,1% by weight of one or more non-carboxylic-ester-linked polyglycol groups each having at least five alkylene oxide units with from two to seven carbon atoms in each alkylene oxide unit, said macromolecule having an average molecular weight of at least 50,000 and a solubility in the lubricating oil of at least 0,5% by weight. The lubricating oil may be a mineral oil, a synthetic hydrocarbon (e.g. a hydrogenated hydrocarbon, polymer, a chlorinated alkane/aryl compound condensation product or a high molecular weight alkylated hydrocarbon such as an alkylated wax), an alkylene oxide polymer or an etherification and/or esterification product thereof, or an ester such as di(2-ethylhexyl) sebacate, tricresyl phosphate or a silicate ester. The macromolecular additive may be a copolymer of (A) an oilsolubilizing olefin of 2-30 carbon atoms or a monomeric compound having a polymerizable ethylenic linkage and containing a hydrocarbyl group of 4-30 aliphatic or cycloaliphatic carbon atoms (e.g. an alkenyl ether, an alkenyl ester of a monocarboxylic acid, or an ester of an unsaturated mono- or di-carboxylic acid), (B) a noncarboxylic-ester-linked polyglycol monomeric compound having a polymerizable ethylenic linkage and a polyglycol group containing at least 5 alkylene oxide units in which each alkylene oxide unit has 2-7 carbon atoms and, optionally, (C) a monomeric polar compound having a polymerizable ethylenic linkage and a polar group (e.g. -COOH, -CONH2, -CONH-ROH or -CONHRNH2 where R is alkylene, carboxyl groups esterified with hydroxy- or amino-substituted alkyl groups, heterocyclic nitrogenous groups, epoxy groups and cyano groups). In monomer (B), the polyvalent linking group or atom between the group bearing the polymerizable ethylenic linkage and the polyglycol group may be -0-, -5-, or a carbonyl, sulphonyloxy, iminocarbonyl, ureylene, iminocarbonyloxy, phosphonyloxy or imino group. Specific examples of monomers (B) are polyglycol amides of unsaturated mono- or dicarboxylic acids and vinyl or allyl monoethers of polyglycols. However, methods other than copolymerization may be used in preparing the macromolecular additive. Specific macromolecular additives mentioned as suitable for addition to mineral lubricating oil are (i) the copolymer of dodecyl methacrylate and methacrylamide-initiated or allylamine-initiated polyethylene glycol, (ii) the copolymer of dodecyl methacrylate and polyethylene glycol monovinyl ether, (iii) the phosphonate product formed by reacting chlorophosphonylated polyisobutylene with the dodecyl mono-ether of polyethylene glycol and (iv) the sulphonate product formed by reacting chlorosulphonylated polyisobutylene with the dodecyl mono-ether of polyethylene glycol. The lubricant composition may contain additional ingredients such as pour point depressants, oiliness and extreme pressure agents, antioxidants and corrosion inhibitors (e.g. P2S5-treated pinene and divalent metal salts of organic dithiophosphoric acids), blooming agents, thickening agents, viscosity improvers (e.g. alkyl methacrylate polymers or butene polymers) or auxiliary detergents and antiwear agents (e.g. alkaline earth phenates of higher alkyl phenols).ALSO:An additive for lubricating oils (see Group III) consists of a predominantly aliphatic or cycloaliphatic macromolecule which comprises up to 99,9% by weight of oil-solubilizing aliphatic or cycloaliphatic hydrocarbon groups and at least 0,1% by weight of one or more non-carboxylic-ester-linked polyglycol groups each having at least 5 alkylene oxide units with 2-7 carbon atoms in each alkylene oxide unit, said macromolecule having an average molecular weight of at least 50,000 and a solubility in the lubricating oil of at least 0,5% by weight. The additive may be a copolymer of (A) an oil-solubilizing olefin of 2-30 carbon atoms or a monomeric compound having a polymerizable ethylenic linkage and containing a hydrocarbyl group of 4-30 aliphatic or cycloaliphatic carbon atoms (e.g. an alkenyl ether, an alkenyl ester of a monocarboxylic acid or an ester of an unsaturated mono- or di-carboxylic acid), (B) a non-carboxylic-ester-linked polyglycol monomeric compound having a polymerizable ethylenic linkage and a polyglycol group containing at least 5 alkylene oxide units in which each alkylene oxide unit has 2-7 carbon atoms and, optionally, (C) a monomeric polar compound having a polymerizable ethylenic linkage and a polar group (e.g. -COOH, -CONH2, -CONHROH or -CONHRNH2 where R is alkylene, carboxyl groups esterified with hydroxy- or amino-substituted alkyl groups, heterocyclic nitrogenous groups, epoxy groups and cyano groups). In monomer (B), the polyvalent linking group or atom between the group bearing the polymerizable ethylenic linkage and the polyglycol group may be -O-, -S-, or a carbonyl, sulphonyloxy, iminocarbonyl, ureylene, imino carbonyloxy, phosphonyloxy or imino group. Specific examples of monomers (B) are polyglycol amides of unsaturated mono- or di-carboxylic acids and vinyl or allyl monoethers of polyglycols. However, methods other than copolymerization may be used in preparing the macromolecular additive. In the examples, the preparation is described of (i) the copolymer of dodecyl methacrylate and methacrylamide-initiated or allylamine-initiated polyethylene glycol, (ii) the copolymer of dodecyl methacrylate and polyethylene glycol monovinyl ether, (iii) the phosphonate product formed by reacting chlorophosphonylated polyisobutylene with the dodecyl mono-ether of polyethelene glycol and (iv) the sulphonate product formed by reacting chlorosulphonylated polyisobutylene with the dodecyl monoether of polyethylene glycol.