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    Composition Containing a Block Copolymer and a Method of Lubricating an Internal Combustion Engine
    1.
    发明申请
    Composition Containing a Block Copolymer and a Method of Lubricating an Internal Combustion Engine 审中-公开
    含有嵌段共聚物的组合物和润滑内燃机的方法

    公开(公告)号：US20110263470A1

    公开(公告)日：2011-10-27

    申请号：US13127114

    申请日：2009-11-03

    申请人： Haihu Qin ,  Ying Wang ,  Marina Baum ,  Jack Kelley ,  Patrick E. Mosier ,  Michael J. Covitch ,  John J. Mullay

    发明人： Haihu Qin ,  Ying Wang ,  Marina Baum ,  Jack Kelley ,  Patrick E. Mosier ,  Michael J. Covitch ,  John J. Mullay

    IPC分类号： C10M145/14

    CPC分类号： C10M149/04 ,  C10M145/14 ,  C10M149/02 ,  C10M149/06 ,  C10M151/02 ,  C10M153/02 ,  C10M2209/084 ,  C10M2217/022 ,  C10M2217/024 ,  C10N2230/26 ,  C10N2240/10 ,  C10N2240/101 ,  C10M2217/02

    摘要： The invention provides a lubricating composition containing an oil of lubricating viscosity and a block copolymer. The block copolymer may contain (a) a hydrophobic first block having C1-30 alkyl (meth)acrylic units, wherein at least 50 wt % of the C1-30 alkyl (meth)acrylic units are C12-15 alkyl (meth)acrylic units, and up to 50 wt % of the C1-30 alkyl (meth)acrylic units are C16 20 alkyl (meth)acrylic units, with the proviso that alkyl groups of the C1-30 alkyl (meth)acrylic units have an average total number of carbon atoms of at least 8; and (b) a second block having (meth)acrylic units further having a heteroatom-containing group providing a polar group. The invention further relates to a method of lubricating an internal combustion engine by lubricating the engine with the lubricating composition. The invention further relates to the use of the block copolymer as an emulsifier and/or pour point depressant.

    摘要翻译： 本发明提供含有润滑粘度油和嵌段共聚物的润滑组合物。 嵌段共聚物可以含有（a）具有（甲基）丙烯酸C 1-30烷基酯单元的疏水性第一嵌段，其中至少50重量％的（甲基）丙烯酸C 1-30烷基酯是C 12-15烷基（甲基）丙烯酸单元 ，最多50重量％的（甲基）丙烯酸C 1-30烷基酯是C 16-20烷基（甲基）丙烯酸单元，条件是（甲基）丙烯酸C 1 -C 30烷基酯的烷基具有平均总数 的碳原子数至少为8; 和（b）具有（甲基）丙烯酸单元的第二嵌段，其进一步具有提供极性基团的含杂原子的基团。 本发明还涉及通过用润滑组合物润滑发动机来润滑内燃机的方法。 本发明还涉及嵌段共聚物作为乳化剂和/或倾点下降剂的用途。

    Lubricant composition
    4.
    发明授权
    Lubricant composition 失效

    公开(公告)号：US2892783A

    公开(公告)日：1959-06-30

    申请号：US72956058

    申请日：1958-04-21

    申请人： CALIFORNIA RESEARCH CORP

    发明人： STUART FRANK A ,  STEWART WILLIAM T ,  KAVANAGH FRANK W

    IPC分类号： C08F8/00 ,  C08F8/14 ,  C08F16/12 ,  C08F20/10 ,  C08F20/58 ,  C08F20/62 ,  C08F22/00 ,  C08F220/18 ,  C08F283/00 ,  C08F283/06 ,  C08F290/06 ,  C08L33/08 ,  C09G1/00 ,  C10M159/00

    CPC分类号： C10M159/005 ,  C08F8/00 ,  C08F16/12 ,  C08F20/58 ,  C08F20/62 ,  C08F22/00 ,  C08F220/18 ,  C08F283/00 ,  C08F283/06 ,  C08F290/062 ,  C08F2800/10 ,  C08F2800/20 ,  C10M1/08 ,  C10M3/00 ,  C10M143/00 ,  C10M143/02 ,  C10M145/02 ,  C10M147/02 ,  C10M149/02 ,  C10M151/02 ,  C10M153/02 ,  C10M2203/02 ,  C10M2203/022 ,  C10M2203/024 ,  C10M2203/04 ,  C10M2203/10 ,  C10M2205/00 ,  C10M2205/02 ,  C10M2205/022 ,  C10M2205/026 ,  C10M2205/14 ,  C10M2205/16 ,  C10M2205/17 ,  C10M2205/18 ,  C10M2205/22 ,  C10M2207/027 ,  C10M2207/282 ,  C10M2207/34 ,  C10M2209/02 ,  C10M2209/084 ,  C10M2209/103 ,  C10M2209/104 ,  C10M2209/105 ,  C10M2209/107 ,  C10M2209/108 ,  C10M2209/109 ,  C10M2213/00 ,  C10M2213/02 ,  C10M2213/04 ,  C10M2213/06 ,  C10M2215/042 ,  C10M2217/00 ,  C10M2217/02 ,  C10M2217/022 ,  C10M2217/023 ,  C10M2217/024 ,  C10M2217/026 ,  C10M2217/028 ,  C10M2217/04 ,  C10M2217/044 ,  C10M2217/045 ,  C10M2217/06 ,  C10M2219/087 ,  C10M2219/088 ,  C10M2219/089 ,  C10M2221/00 ,  C10M2221/02 ,  C10M2221/04 ,  C10M2221/041 ,  C10M2221/043 ,  C10M2223/041 ,  C10M2223/045 ,  C10M2223/12 ,  C10M2225/00 ,  C10M2225/02 ,  C10M2225/04 ,  C10M2227/02 ,  C10M2229/00 ,  C10N2210/02 ,  C10N2240/04 ,  C10N2240/042 ,  C10N2240/044 ,  C10N2240/046 ,  C10N2240/10 ,  C10N2240/101 ,  C10N2240/104 ,  C10N2240/106 ,  C10N2270/02 ,  Y10S526/933 ,  C08F8/14 ,  C08F8/12 ,  C08F120/18 ,  C08F110/10

    摘要： A lubricating composition, especially suitable for use in internal combustion engines, comprises a major proportion by weight of a lubricating oil and a minor proportion by weight, sufficient to enhance the detergent characteristics of the composition, of an additive consisting of a predominantly aliphatic or cycloaliphatic macromolecule, which macromolecule comprises up to 99,9% by weight of oil-solubilizing aliphatic or cycloaliphatic hydrocarbon groups and at least 0,1% by weight of one or more non-carboxylic-ester-linked polyglycol groups each having at least five alkylene oxide units with from two to seven carbon atoms in each alkylene oxide unit, said macromolecule having an average molecular weight of at least 50,000 and a solubility in the lubricating oil of at least 0,5% by weight. The lubricating oil may be a mineral oil, a synthetic hydrocarbon (e.g. a hydrogenated hydrocarbon, polymer, a chlorinated alkane/aryl compound condensation product or a high molecular weight alkylated hydrocarbon such as an alkylated wax), an alkylene oxide polymer or an etherification and/or esterification product thereof, or an ester such as di(2-ethylhexyl) sebacate, tricresyl phosphate or a silicate ester. The macromolecular additive may be a copolymer of (A) an oilsolubilizing olefin of 2-30 carbon atoms or a monomeric compound having a polymerizable ethylenic linkage and containing a hydrocarbyl group of 4-30 aliphatic or cycloaliphatic carbon atoms (e.g. an alkenyl ether, an alkenyl ester of a monocarboxylic acid, or an ester of an unsaturated mono- or di-carboxylic acid), (B) a noncarboxylic-ester-linked polyglycol monomeric compound having a polymerizable ethylenic linkage and a polyglycol group containing at least 5 alkylene oxide units in which each alkylene oxide unit has 2-7 carbon atoms and, optionally, (C) a monomeric polar compound having a polymerizable ethylenic linkage and a polar group (e.g. -COOH, -CONH2, -CONH-ROH or -CONHRNH2 where R is alkylene, carboxyl groups esterified with hydroxy- or amino-substituted alkyl groups, heterocyclic nitrogenous groups, epoxy groups and cyano groups). In monomer (B), the polyvalent linking group or atom between the group bearing the polymerizable ethylenic linkage and the polyglycol group may be -0-, -5-, or a carbonyl, sulphonyloxy, iminocarbonyl, ureylene, iminocarbonyloxy, phosphonyloxy or imino group. Specific examples of monomers (B) are polyglycol amides of unsaturated mono- or dicarboxylic acids and vinyl or allyl monoethers of polyglycols. However, methods other than copolymerization may be used in preparing the macromolecular additive. Specific macromolecular additives mentioned as suitable for addition to mineral lubricating oil are (i) the copolymer of dodecyl methacrylate and methacrylamide-initiated or allylamine-initiated polyethylene glycol, (ii) the copolymer of dodecyl methacrylate and polyethylene glycol monovinyl ether, (iii) the phosphonate product formed by reacting chlorophosphonylated polyisobutylene with the dodecyl mono-ether of polyethylene glycol and (iv) the sulphonate product formed by reacting chlorosulphonylated polyisobutylene with the dodecyl mono-ether of polyethylene glycol. The lubricant composition may contain additional ingredients such as pour point depressants, oiliness and extreme pressure agents, antioxidants and corrosion inhibitors (e.g. P2S5-treated pinene and divalent metal salts of organic dithiophosphoric acids), blooming agents, thickening agents, viscosity improvers (e.g. alkyl methacrylate polymers or butene polymers) or auxiliary detergents and antiwear agents (e.g. alkaline earth phenates of higher alkyl phenols).ALSO:An additive for lubricating oils (see Group III) consists of a predominantly aliphatic or cycloaliphatic macromolecule which comprises up to 99,9% by weight of oil-solubilizing aliphatic or cycloaliphatic hydrocarbon groups and at least 0,1% by weight of one or more non-carboxylic-ester-linked polyglycol groups each having at least 5 alkylene oxide units with 2-7 carbon atoms in each alkylene oxide unit, said macromolecule having an average molecular weight of at least 50,000 and a solubility in the lubricating oil of at least 0,5% by weight. The additive may be a copolymer of (A) an oil-solubilizing olefin of 2-30 carbon atoms or a monomeric compound having a polymerizable ethylenic linkage and containing a hydrocarbyl group of 4-30 aliphatic or cycloaliphatic carbon atoms (e.g. an alkenyl ether, an alkenyl ester of a monocarboxylic acid or an ester of an unsaturated mono- or di-carboxylic acid), (B) a non-carboxylic-ester-linked polyglycol monomeric compound having a polymerizable ethylenic linkage and a polyglycol group containing at least 5 alkylene oxide units in which each alkylene oxide unit has 2-7 carbon atoms and, optionally, (C) a monomeric polar compound having a polymerizable ethylenic linkage and a polar group (e.g. -COOH, -CONH2, -CONHROH or -CONHRNH2 where R is alkylene, carboxyl groups esterified with hydroxy- or amino-substituted alkyl groups, heterocyclic nitrogenous groups, epoxy groups and cyano groups). In monomer (B), the polyvalent linking group or atom between the group bearing the polymerizable ethylenic linkage and the polyglycol group may be -O-, -S-, or a carbonyl, sulphonyloxy, iminocarbonyl, ureylene, imino carbonyloxy, phosphonyloxy or imino group. Specific examples of monomers (B) are polyglycol amides of unsaturated mono- or di-carboxylic acids and vinyl or allyl monoethers of polyglycols. However, methods other than copolymerization may be used in preparing the macromolecular additive. In the examples, the preparation is described of (i) the copolymer of dodecyl methacrylate and methacrylamide-initiated or allylamine-initiated polyethylene glycol, (ii) the copolymer of dodecyl methacrylate and polyethylene glycol monovinyl ether, (iii) the phosphonate product formed by reacting chlorophosphonylated polyisobutylene with the dodecyl mono-ether of polyethelene glycol and (iv) the sulphonate product formed by reacting chlorosulphonylated polyisobutylene with the dodecyl monoether of polyethylene glycol.

    LUBRICANT COMPOSITION WITH PHOSPHORUS-FUNCTIONALIZED POLYMERS
    5.
    发明申请
    LUBRICANT COMPOSITION WITH PHOSPHORUS-FUNCTIONALIZED POLYMERS 有权
    具有磷官能化聚合物的润滑剂组合物

    公开(公告)号：US20140135242A1

    公开(公告)日：2014-05-15

    申请号：US14119550

    申请日：2012-04-19

    申请人： Boris Eisenberg ,  Ellen Suchert

    发明人： Boris Eisenberg ,  Ellen Suchert

    IPC分类号： C10M153/02

    CPC分类号： C10M153/02 ,  C10M2203/1006 ,  C10M2203/1025 ,  C10M2205/0285 ,  C10M2209/084 ,  C10M2223/04 ,  C10M2223/045 ,  C10M2223/047 ,  C10M2223/049 ,  C10M2223/06 ,  C10M2225/02 ,  C10N2220/021 ,  C10N2230/06 ,  C10N2230/08 ,  C10N2240/04 ,  C10N2240/10 ,  C10N2220/022

    摘要： The present invention relates to a lubricant composition comprising at least one polyalkyl(meth)acrylate including repeating units derived from (meth)acrylates having 6 to 22 carbon atoms in the alcohol radical, wherein the polyalkyl(meth)acrylate includes repeating units derived from ethylenically unsaturated monomers having at least one covalently bonded phosphorus atom. The present invention further relates to a polyalkyl(meth)acrylate suitable for such a lubricant composition and to the use of a polyalkyl(meth)acrylate having repeating units derived from ethylenically unsaturated monomers having at least one covalently bonded phosphorus atom for reducing friction.

    摘要翻译： 本发明涉及包含至少一种（甲基）丙烯酸烷基酯（包括衍生自醇基中具有6-22个碳原子的（甲基）丙烯酸酯）的重复单元）的润滑剂组合物，其中（甲基）丙烯酸烷基酯包括衍生自烯属的 具有至少一个共价键合的磷原子的不饱和单体。 本发明还涉及适用于这种润滑剂组合物的聚（甲基）丙烯酸烷基酯，以及具有衍生自具有至少一个共价键合的磷原子的具有至少一个共价键的磷原子的重复单元的（甲基）丙烯酸烷基酯的（甲基）丙烯酸烷基酯用于减少摩擦。