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公开(公告)号：US09403149B2
公开(公告)日：2016-08-02
申请号：US13238332
申请日：2011-09-21
申请人： Wayne Turbeville , Greg Korynta
发明人： Wayne Turbeville , Greg Korynta
IPC分类号： B01J21/02 , B01J27/14 , B01J27/16 , B01J35/00 , B01J35/02 , B01J21/08 , B01J37/03 , B01J37/08 , B01J23/20 , B01J27/18 , B01J27/182 , B01J37/00
CPC分类号： B01J21/08 , B01J23/20 , B01J27/18 , B01J27/182 , B01J35/0013 , B01J37/0018 , B01J37/038 , B01J37/08 , B01J2523/00 , B01J2523/41 , B01J2523/51 , B01J2523/56
摘要： The present invention relates to solid phosphoric acid (SPA) catalysts, processes for making the catalysts, and processes for conversion of hydrocarbons using the catalysts, such as oligomerization of propylene. In an exemplary embodiment, the catalyst comprises a calcined extrudate of phosphoric acid, diatomaceous earth, and niobic acid. Methods for converting hydrocarbons to olefins comprise contacting a hydrocarbon feedstock with the catalyst at hydrocarbon conversion conditions.
摘要翻译： 本发明涉及固体磷酸（SPA）催化剂，制备催化剂的方法，以及使用催化剂转化烃的方法，例如丙烯的低聚。 在一个示例性实施方案中，催化剂包括磷酸，硅藻土和铌酸的煅烧挤出物。 将烃转化为烯烃的方法包括在烃转化条件下使烃原料与催化剂接触。
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公开(公告)号：US20090005623A1
公开(公告)日：2009-01-01
申请号：US11770767
申请日：2007-06-29
IPC分类号： B01J27/182 , C07C2/00
CPC分类号： B01J27/182 , B01J35/002 , B01J35/1038 , B01J35/1076 , B01J35/108 , B01J37/0009 , B01J37/0018 , C07C2/18 , C07C2/70 , C07C2527/173 , C10G29/02 , C10G29/205 , C10G50/00
摘要： The present invention relates to a solid phosphoric acid catalyst and a process for conversion of hydrocarbons using a solid phosphoric acid catalyst. The solid phosphoric acid catalyst comprises silicon orthophosphate, and has a silicon orthophosphate to silicon pyrophosphate ratio of at least about 5:1. The total pore volume of the solid phosphoric acid catalyst is at least about 0.17 cm3 per gram of catalyst, of which at least about 0.15 cm3 per gram is contributed by pores with diameter of at least about 10,000 Å.
摘要翻译： 本发明涉及固体磷酸催化剂和使用固体磷酸催化剂转化烃的方法。 固体磷酸催化剂包括正磷酸硅，并且具有至少约5:1的正磷酸硅与焦磷酸硅的比例。 固体磷酸催化剂的总孔体积为每克催化剂至少约0.17cm 3，其中至少约0.15cm 3 /克由具有至少约10,000埃的直径的孔贡献。
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公开(公告)号：US08063260B2
公开(公告)日：2011-11-22
申请号：US12499082
申请日：2009-07-07
CPC分类号： B01J27/182 , B01J35/002 , B01J35/1038 , B01J35/1076 , B01J35/108 , B01J37/0009 , B01J37/0018 , C07C2/18 , C07C2/70 , C07C2527/173 , C10G29/02 , C10G29/205 , C10G50/00
摘要： The present invention relates to a solid phosphoric acid catalyst and a process for conversion of hydrocarbons using a solid phosphoric acid catalyst. The solid phosphoric acid catalyst comprises silicon orthophosphate, and has a silicon orthophosphate to silicon pyrophosphate ratio of at least about 5:1. The total pore volume of the solid phosphoric acid catalyst is at least about 0.17 cm3 per gram of catalyst, of which at least about 0.15 cm3 per gram is contributed by pores with diameter of at least about 10,000 Å.
摘要翻译： 本发明涉及固体磷酸催化剂和使用固体磷酸催化剂转化烃的方法。 固体磷酸催化剂包括正磷酸硅，并且具有至少约5:1的正磷酸硅与焦磷酸硅的比例。 固体磷酸催化剂的总孔体积为每克催化剂至少约0.17cm 3，其中至少约0.15cm 3 /克由具有至少约10,000埃的直径的孔贡献。
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公开(公告)号：US20100069692A1
公开(公告)日：2010-03-18
申请号：US12499082
申请日：2009-07-07
IPC分类号： C07C5/03 , B01J27/182
CPC分类号： B01J27/182 , B01J35/002 , B01J35/1038 , B01J35/1076 , B01J35/108 , B01J37/0009 , B01J37/0018 , C07C2/18 , C07C2/70 , C07C2527/173 , C10G29/02 , C10G29/205 , C10G50/00
摘要： The present invention relates to a solid phosphoric acid catalyst and a process for conversion of hydrocarbons using a solid phosphoric acid catalyst. The solid phosphoric acid catalyst comprises silicon orthophosphate, and has a silicon orthophosphate to silicon pyrophosphate ratio of at least about 5:1. The total pore volume of the solid phosphoric acid catalyst is at least about 0.17 cm3 per gram of catalyst, of which at least about 0.15 cm3 per gram is contributed by pores with diameter of at least about 10,000 Å.
摘要翻译： 本发明涉及固体磷酸催化剂和使用固体磷酸催化剂转化烃的方法。 固体磷酸催化剂包括正磷酸硅，并且具有至少约5:1的正磷酸硅与焦磷酸硅的比例。 固体磷酸催化剂的总孔体积为每克催化剂至少约0.17cm 3，其中至少约0.15cm 3 /克由具有至少约10,000埃的直径的孔贡献。
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公开(公告)号：US20070034552A1
公开(公告)日：2007-02-15
申请号：US11203915
申请日：2005-08-15
申请人： Wayne Turbeville , Nora Yap , Yeping Cai , Jurgen Ladebeck
发明人： Wayne Turbeville , Nora Yap , Yeping Cai , Jurgen Ladebeck
CPC分类号： C10G25/003 , B01J20/06 , B01J23/007 , B01J23/80
摘要： The present invention is a method for the adsorption of sulfur-containing compounds from a hydrocarbon feedstream, and in particular, an olefin feedstream. The method comprises contacting the sulfur-containing compound with a copper oxide/zinc oxide/aluminum oxide catalyst optionally promoted with a metal.
摘要翻译： 本发明是从烃类原料流，特别是烯烃原料流中吸附含硫化合物的方法。 该方法包括使含硫化合物与任选被金属促进的氧化铜/氧化锌/氧化铝催化剂接触。
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公开(公告)号：US09278346B2
公开(公告)日：2016-03-08
申请号：US13557475
申请日：2012-07-25
申请人： Wenqin Shen , Alguo Liu , Wayne Turbeville
发明人： Wenqin Shen , Alguo Liu , Wayne Turbeville
IPC分类号： B01J23/44 , B01J23/42 , B01J35/00 , B01J37/02 , B01J23/847 , B01J23/889 , B01J21/06 , B01J23/14 , B01J23/28 , B01J23/36 , B01J23/46 , B01J23/63 , B01J23/648 , B01J23/652 , B01J23/656 , B01J23/72 , B01J23/75 , B01J23/755 , B01J23/83 , B01J23/882 , B01J23/883 , B01J23/888 , B01J37/00 , C10L1/04 , C10G3/00
CPC分类号： B01J35/002 , B01J21/066 , B01J23/14 , B01J23/28 , B01J23/36 , B01J23/42 , B01J23/44 , B01J23/462 , B01J23/464 , B01J23/466 , B01J23/468 , B01J23/63 , B01J23/6482 , B01J23/6484 , B01J23/6486 , B01J23/6525 , B01J23/6527 , B01J23/6562 , B01J23/6567 , B01J23/72 , B01J23/75 , B01J23/755 , B01J23/83 , B01J23/8472 , B01J23/8474 , B01J23/8476 , B01J23/882 , B01J23/883 , B01J23/888 , B01J23/8892 , B01J23/8896 , B01J37/0009 , B01J37/0207 , B01J37/0242 , C10G3/47 , C10G3/48 , C10G3/52 , C10G2300/1011 , C10G2300/1014 , C10G2300/1018 , C10L1/04 , Y02P30/20
摘要： A hydrodeoxygenation catalyst comprises a metal catalyst, an acid promoter, and a support. The metal catalyst is selected from platinum, palladium, ruthenium, rhenium rhodium, osmium, iridium, nickel, cobalt, molybdenum, copper, tin, or mixtures thereof. The support is a promoted-zirconium material including texture promoters and acid promoters. The hydrodeoxygenation catalyst may be used for hydrodeoxygenation (HDO) of sugar or sugar alcohol in an aqueous solution. In one embodiment the HDO catalyst may be used for HDO of fatty acids such as fatty acid methyl esters (FAME), triglycerols (in plant oil and animal fat), pyrolysis oil, or lignin. The hydrodeoxygenation catalyst for fatty acid process does not require the use of an acid promoter, it is optional.
摘要翻译： 加氢脱氧催化剂包括金属催化剂，酸促进剂和载体。 金属催化剂选自铂，钯，钌，铑铑，锇，铱，镍，钴，钼，铜，锡或其混合物。 载体是促进锆材料，包括纹理启动子和酸促进剂。 加氢脱氧催化剂可用于水溶液中糖或糖醇的加氢脱氧（HDO）。 在一个实施方案中，HDO催化剂可用于脂肪酸的HDO，例如脂肪酸甲酯（FAME），甘油三酯（植物油和动物脂肪），热解油或木质素。 用于脂肪酸方法的加氢脱氧催化剂不需要使用酸促进剂，它是任选的。
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公开(公告)号：US20140031546A1
公开(公告)日：2014-01-30
申请号：US13557475
申请日：2012-07-25
申请人： Wenqin Shen , Alguo Liu , Wayne Turbeville
发明人： Wenqin Shen , Alguo Liu , Wayne Turbeville
IPC分类号： B01J23/755 , B01J23/44 , B01J23/46 , B01J23/42 , B01J23/24 , B01J23/72 , B01J23/20 , B01J23/10 , B01J23/32 , B01J23/75 , C07C29/132 , C07C51/00 , C07C45/00 , C07D475/00 , C07C1/22
CPC分类号： B01J35/002 , B01J21/066 , B01J23/14 , B01J23/28 , B01J23/36 , B01J23/42 , B01J23/44 , B01J23/462 , B01J23/464 , B01J23/466 , B01J23/468 , B01J23/63 , B01J23/6482 , B01J23/6484 , B01J23/6486 , B01J23/6525 , B01J23/6527 , B01J23/6562 , B01J23/6567 , B01J23/72 , B01J23/75 , B01J23/755 , B01J23/83 , B01J23/8472 , B01J23/8474 , B01J23/8476 , B01J23/882 , B01J23/883 , B01J23/888 , B01J23/8892 , B01J23/8896 , B01J37/0009 , B01J37/0207 , B01J37/0242 , C10G3/47 , C10G3/48 , C10G3/52 , C10G2300/1011 , C10G2300/1014 , C10G2300/1018 , C10L1/04 , Y02P30/20
摘要： A hydrodeoxygenation catalyst comprises a metal catalyst, an acid promoter, and a support. The metal catalyst is selected from platinum, palladium, ruthenium, rhenium rhodium, osmium, iridium, nickel, cobalt, molybdenum, copper, tin, or mixtures thereof. The support is a promoted-zirconium material including texture promoters and acid promoters. The hydrodeoxygenation catalyst may be used for hydrodeoxygenation (HDO) of sugar or sugar alcohol in an aqueous solution. In one embodiment the HDO catalyst may be used for HDO of fatty acids such as fatty acid methyl esters (FAME), triglycerols (in plant oil and animal fat), pyrolysis oil, or lignin. The hydrodeoxygenation catalyst for fatty acid process does not require the use of an acid promoter, it is optional.
摘要翻译： 加氢脱氧催化剂包括金属催化剂，酸促进剂和载体。 金属催化剂选自铂，钯，钌，铑铑，锇，铱，镍，钴，钼，铜，锡或其混合物。 载体是促进锆材料，包括纹理启动子和酸促进剂。 加氢脱氧催化剂可用于水溶液中糖或糖醇的加氢脱氧（HDO）。 在一个实施方案中，HDO催化剂可用于脂肪酸的HDO，例如脂肪酸甲酯（FAME），甘油三酯（植物油和动物脂肪），热解油或木质素。 用于脂肪酸方法的加氢脱氧催化剂不需要使用酸促进剂，这是任选的。
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公开(公告)号：US20110301021A1
公开(公告)日：2011-12-08
申请号：US13201892
申请日：2010-03-03
申请人： Aiguo Liu , Todd J. Cole, II , Wayne Turbeville
发明人： Aiguo Liu , Todd J. Cole, II , Wayne Turbeville
IPC分类号： B01J21/06 , B01J27/135 , B01J27/25 , B01J31/34 , B01J31/38 , B01J27/02 , B01J23/28 , B01J23/30 , B01J32/00 , B01J35/10 , B01J27/18 , B01J35/02 , B01J23/26
CPC分类号： B01J37/0009 , B01J21/066 , B01J23/26 , B01J23/28 , B01J23/30 , B01J23/866 , B01J23/868 , B01J35/002 , B01J35/1014 , B01J35/1019 , B01J37/031 , C07C29/00 , C07C29/60 , Y02P20/52 , C07C31/202 , C07C31/205 , C07C31/225
摘要： A polyacid-promoted, zirconia catalyst or catalyst support having a high crush strength, surface area and pore volume is described. The polyacid-promoted, zirconia catalyst or catalyst support may be made by combining a zirconium compound with a polyacid/promoter material that includes the group 6 metals (i.e., chromium (Cr), molybdenum (Mo), tungsten (W)), as well as phosphoric acids, sulfuric acids, and polyorganic acids. The zirconyl-promoter precursor may be extruded in the absence of any binder or extrusion aid. The polyacid-promoted, zirconia catalyst or catalyst support is hydrothermally stable in aqueous phase hydrogenation or hydrogenoloysis reactions.
摘要翻译： 描述了具有高抗压强度，表面积和孔体积的多酸促进的氧化锆催化剂或催化剂载体。 多酸促进的氧化锆催化剂或催化剂载体可以通过将锆化合物与包含第6族金属（即，铬（Cr），钼（Mo），钨（W））的多元酸/促进剂材料组合来制备，如 以及磷酸，硫酸和聚有机酸。 在不存在任何粘合剂或挤出助剂的情况下，可以将锆基 - 促进剂前体挤出。 多酸促进的氧化锆催化剂或催化剂载体在水相氢化或氢化反应中是水热稳定的。
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公开(公告)号：US20130072735A1
公开(公告)日：2013-03-21
申请号：US13238332
申请日：2011-09-21
申请人： Wayne Turbeville , Greg Korynta
发明人： Wayne Turbeville , Greg Korynta
IPC分类号： C07C2/66 , B01J27/19 , B01J27/182 , B01J21/16 , B01J27/199 , B01J27/198 , B01J21/02 , B01J27/188 , C07C2/24
CPC分类号： B01J21/08 , B01J23/20 , B01J27/18 , B01J27/182 , B01J35/0013 , B01J37/0018 , B01J37/038 , B01J37/08 , B01J2523/00 , B01J2523/41 , B01J2523/51 , B01J2523/56
摘要： The present invention relates to solid phosphoric acid (SPA) catalysts, processes for making the catalysts, and processes for conversion of hydrocarbons using the catalysts, such as oligomerization of propylene. In an exemplary embodiment, the catalyst comprises a calcined extrudate of phosphoric acid, diatomaceous earth, and niobic acid. Methods for converting hydrocarbons to olefins comprise contacting a hydrocarbon feedstock with the catalyst at hydrocarbon conversion conditions.
摘要翻译： 本发明涉及固体磷酸（SPA）催化剂，制备催化剂的方法，以及使用催化剂转化烃的方法，例如丙烯的低聚。 在一个示例性实施方案中，催化剂包括磷酸，硅藻土和铌酸的煅烧挤出物。 将烃转化为烯烃的方法包括在烃转化条件下使烃原料与催化剂接触。
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公开(公告)号：US07557060B2
公开(公告)日：2009-07-07
申请号：US11770767
申请日：2007-06-29
IPC分类号： B01J27/00 , B01J27/182 , B01J21/00 , C01B15/16 , C01B25/26 , C07C2/02 , C07C6/12 , C07C13/28 , C07C2/64 , C07C15/067
CPC分类号： B01J27/182 , B01J35/002 , B01J35/1038 , B01J35/1076 , B01J35/108 , B01J37/0009 , B01J37/0018 , C07C2/18 , C07C2/70 , C07C2527/173 , C10G29/02 , C10G29/205 , C10G50/00
摘要： The present invention relates to a solid phosphoric acid catalyst and a process for conversion of hydrocarbons using a solid phosphoric acid catalyst. The solid phosphoric acid catalyst comprises silicon orthophosphate, and has a silicon orthophosphate to silicon pyrophosphate ratio of at least about 5:1. The total pore volume of the solid phosphoric acid catalyst is at least about 0.17 cm3 per gram of catalyst, of which at least about 0.15 cm3 per gram is contributed by pores with diameter of at least about 10,000 Å.
摘要翻译： 本发明涉及固体磷酸催化剂和使用固体磷酸催化剂转化烃的方法。 固体磷酸催化剂包括正磷酸硅，并且具有至少约5:1的正磷酸硅与焦磷酸硅的比例。 固体磷酸催化剂的总孔体积为每克催化剂至少约0.17cm 3，其中至少约0.15cm 3 /克由具有至少约10,000埃的直径的孔贡献。
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