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    Electrochemical synthesis of ammonia
    1.
    发明授权
    Electrochemical synthesis of ammonia 失效
    电化学合成氨

    公开(公告)号：US07314544B2

    公开(公告)日：2008-01-01

    申请号：US11212038

    申请日：2005-08-25

    申请人： Oliver J. Murphy ,  Adrian J. Denvir ,  Sorin G. Teodorescu ,  Kyle B. Uselton

    发明人： Oliver J. Murphy ,  Adrian J. Denvir ,  Sorin G. Teodorescu ,  Kyle B. Uselton

    IPC分类号： C25B1/00

    CPC分类号： C25B1/00

    摘要： A method for the anodic electrochemical synthesis of ammonia gas. The method comprises providing an electrolyte between an anode and a cathode, providing nitrogen and hydrogen gases to the cathode, oxidizing negatively charged nitrogen-containing species and negatively charged hydrogen-containing species present in the electrolyte at the anode to form adsorbed nitrogen species and adsorbed hydrogen species, respectively, and reacting the adsorbed nitrogen species with the adsorbed hydrogen species to form ammonia. Nitrogen and hydrogen gases may be provided through a porous cathode substrate. The negatively charged nitrogen-containing species in the electrolyte may be produced by reducing nitrogen gas at the cathode and/or by supplying a nitrogen-containing salt, such as lithium nitride, into the molten salt electrolyte. Similarly, the negatively charged hydrogen-containing species in the electrolyte may be produced by reducing hydrogen gas at the cathode and/or by supplying a hydrogen-containing salt, such as lithium hydride, into the molten salt electrolyte.

    摘要翻译： 一种用于阳极电化学合成氨气的方法。 该方法包括在阳极和阴极之间提供电解质，向阴极提供氮气和氢气，在阳极处氧化带负电荷的含氮物质和存在于电解质中的带负电荷的含氢物质以形成吸附的氮物质并吸附 氢物种，并将吸附的氮物质与吸附的氢物质反应形成氨。 可以通过多孔阴极基底提供氮气和氢气。 电解质中带负电的含氮物质可以通过在阴极处还原氮气和/或通过向熔融盐电解质中提供氮化钠等含氮盐来制备。 类似地，电解质中带负电荷的含氢物质可以通过还原阴极处的氢气和/或通过向熔融盐电解质中提供氢化锂等含氢盐来制备。

    Electrochemical synthesis of ammonia
    2.
    发明授权
    Electrochemical synthesis of ammonia 失效
    电化学合成氨

    公开(公告)号：US06881308B2

    公开(公告)日：2005-04-19

    申请号：US10090444

    申请日：2002-03-04

    申请人： Adrian J. Denvir ,  Oliver J. Murphy ,  Alan J. Cisar ,  Priscilla Robertson ,  Kyle Uselton

    发明人： Adrian J. Denvir ,  Oliver J. Murphy ,  Alan J. Cisar ,  Priscilla Robertson ,  Kyle Uselton

    IPC分类号： C25B1/00 ,  C25B9/06 ,  C25B3/02 ,  C25B9/18

    CPC分类号： C25B1/00

    摘要： A method for electrochemical synthesis of ammonia gas comprising providing an electrolyte between an anode and a cathode, providing hydrogen gas to the anode, oxidizing negatively charged nitrogen-containing species present in the electrolyte at the anode to form an adsorbed nitrogen species, and reacting the hydrogen with the adsorbed nitrogen species to form ammonia. Preferably, the hydrogen gas is provided to the anode by passing the hydrogen gas through a porous anode substrate. It is also preferred to produce the negatively charged nitrogen-containing species in the electrolyte by reducing nitrogen gas at the cathode. However, the negatively charged nitrogen-containing species may also be provided by supplying a nitrogen-containing salt, such as lithium nitride, into the molten salt electrolyte mixture in a sufficient amount to provide some or all of the nitrogen consumed in the production of ammonia.

    摘要翻译： 一种用于电化学合成氨气的方法，包括在阳极和阴极之间提供电解质，向阳极提供氢气，在阳极处氧化存在于电解质中的带负电荷的含氮物质以形成吸附的氮物质，并使 氢与吸附的氮物质形成氨。 优选地，通过使氢气通过多孔阳极基板而将氢气提供给阳极。 还优选通过还原阴极处的氮气来在电解质中产生带负电的含氮物质。 然而，带负电的含氮物质也可以通过向熔融盐电解质混合物中提供足够量的含氮盐（例如氮化钠）来提供在氨生产中消耗的一部分或全部氮 。

    Water sources for automotive devices
    9.
    发明授权
    Water sources for automotive devices 失效
    汽车设备用水源

    公开(公告)号：US06804949B2

    公开(公告)日：2004-10-19

    申请号：US10226361

    申请日：2002-08-22

    申请人： Craig C. Andrews ,  Alan J. Cisar ,  Carlos Salinas ,  Oliver J. Murphy ,  A. John Appleby

    发明人： Craig C. Andrews ,  Alan J. Cisar ,  Carlos Salinas ,  Oliver J. Murphy ,  A. John Appleby

    IPC分类号： F01N300

    CPC分类号： C25B15/08 ,  F01N2240/22 ,  F02B43/10 ,  F02B47/02 ,  F02B2043/106 ,  Y02T10/121 ,  Y02T10/32 ,  Y02T90/42

    摘要： The present invention provides a self-replenishing liquid water source onboard an automobile for supplying liquid water to an electrolyzer, such as an on-board hydrogen generator useful for the suppression of unwanted emissions. While automobiles typically have water reservoirs resupplied by a person, the invention provides a passive means of water collection for reliable replenishment due to operations of the automobile itself. The invention provides condensate from the engine exhaust gas by cooling a region of the exhaust system using cooling fluid from the engine coolant system. The cooling fluid is circulated during a period following the engine cold start event when the heat load on the engine coolant system is low.

    摘要翻译： 本发明提供了一种用于向电解器供应液体水的汽车上的自补充液体水源，例如可用于抑制不期望的排放物的板上氢气发生器。 虽然汽车通常具有由人员补充的储水器，但是由于汽车本身的操作，本发明提供了一种被动的水收集装置，用于可靠的补给。 本发明通过使用来自发动机冷却剂系统的冷却流体冷却排气系统的区域来提供来自发动机废气的冷凝物。 当发动机冷启动事件发动机冷却系统的热负荷低时，冷却液循环。