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    Compositions containing copolymers of olefinic monomers
    2.
    发明授权
    Compositions containing copolymers of olefinic monomers 失效
    含有烯属单体共聚物的组合物

    公开(公告)号：US07619040B2

    公开(公告)日：2009-11-17

    申请号：US11116706

    申请日：2005-04-28

    申请人： Steven V. Barancyk ,  Simion Coca ,  Edward R. Coleridge ,  Gregory J. McCollum ,  James B. O'Dwyer

    发明人： Steven V. Barancyk ,  Simion Coca ,  Edward R. Coleridge ,  Gregory J. McCollum ,  James B. O'Dwyer

    IPC分类号： C08F8/32

    CPC分类号： C08F8/00 ,  B05D1/007 ,  B05D3/0209 ,  B05D3/067 ,  B05D7/53 ,  B05D7/57 ,  C08F210/10 ,  C08F220/10 ,  C09D123/22 ,  C08F210/00 ,  C08F220/12 ,  C08L2666/28

    摘要： A composition that includes a non-gelled copolymer that contains residues having structural units (I): where n is an integer from 1 to 10,000; R1 is linear or branched C1 to C4 alkyl; R2 is selected from the group consisting of methyl, linear, cyclic or branched C2 to C20 alkyl, alkenyl, aryl, alkaryl and aralkyl, and R3 is a group resulting from a post polymerization reaction selected from transesterification, transamidification and hydrolysis with a compound selected from hydroxy functional compounds and amine functional compounds. The composition may contain co-reactive functional groups and may be a thermosetting composition. A substrate may be coated with the thermosetting composition singly or as part of a multi-layer composite coating that includes a base coat layer and a substantially pigment free top coat layer.

    摘要翻译： 包含含有具有结构单元（I）的残基的非胶凝共聚物的组合物：其中n为1至10,000的整数; R1是直链或支链C1-C4烷基; R 2选自甲基，直链，环状或支链C 2至C 20烷基，烯基，芳基，烷芳基和芳烷基，并且R 3是由选择酯交换，转酰胺化和水解的后聚合反应得到的基团， 由羟基官能化合物和胺官能化合物组成。 组合物可以含有共反应性官能团并且可以是热固性组合物。 基材可以单独地涂覆有热固性组合物，或者作为多层复合涂层的一部分，其包括底涂层和基本上不含颜料的顶涂层。

    Amide functional monomers
    3.
    发明授权
    Amide functional monomers 失效
    酰胺官能单体

    公开(公告)号：US6005065A

    公开(公告)日：1999-12-21

    申请号：US138255

    申请日：1998-08-21

    申请人： Steven V. Barancyk ,  Neil D. McMurdie ,  James B. O'Dwyer

    发明人： Steven V. Barancyk ,  Neil D. McMurdie ,  James B. O'Dwyer

    IPC分类号： C07C235/06 ,  C08F20/36 ,  C08G73/00 ,  C07C229/00 ,  C08G69/00

    CPC分类号： C07C235/06 ,  C08F20/36

    摘要： Ethylenically unsaturated compounds are provided having the structure: ##STR1## wherein R.sub.1 is hydrogen or methyl, R.sub.2 is a divalent linking group having 2 to 20 carbon atoms such as alkylene groups, and R.sub.3 is hydrogen or lower alkyl having 1 to 4 carbon atoms, and when R.sub.3 is hydrogen and R.sub.2 has two carbon atoms R.sub.2 is methyl methylene.

    摘要翻译： 提供具有以下结构的烯键式不饱和化合物：其中R1是氢或甲基，R2是具有2至20个碳原子的二价连接基团，例如亚烷基，R 3是氢或具有1至4个碳原子的低级烷基，当R 3 是氢，R2有两个碳原子，R2是甲基亚甲基。

    Coating compositions comprising silyl blocked components, coatings, coated substrates and methods related thereto
    4.
    发明授权
    Coating compositions comprising silyl blocked components, coatings, coated substrates and methods related thereto 失效
    包含甲硅烷基封端组分，涂层，涂覆基材和与其有关的方法的涂料组合物

    公开(公告)号：US07172809B2

    公开(公告)日：2007-02-06

    申请号：US10642826

    申请日：2003-08-19

    申请人： Steven V. Barancyk ,  John W. Burgman ,  James B. O'Dywer ,  Laura A. Kiefer-Liptak ,  Michael Allen Mayo ,  Gregory J. McCollum ,  Shiryn Tyebjee

    发明人： Steven V. Barancyk ,  John W. Burgman ,  James B. O'Dywer ,  Laura A. Kiefer-Liptak ,  Michael Allen Mayo ,  Gregory J. McCollum ,  Shiryn Tyebjee

    IPC分类号： B32B5/16

    CPC分类号： C09D201/06 ,  C08G18/4692 ,  C08G18/792 ,  C09D167/00 ,  C09D175/04 ,  Y10T428/25 ,  Y10T428/251 ,  Y10T428/254 ,  Y10T428/2991 ,  Y10T428/2993 ,  Y10T428/2998 ,  Y10T428/31511 ,  Y10T428/31551 ,  C08L2666/28 ,  C08L2666/16

    摘要： Coating compositions formed from at least one hydroxyl functional non-vinyl material comprising at least one alcoholic hydroxyl group blocked with a hydrolyzable silyl group, and at least one curing agent are provided by the present invention. Another embodiment of the present invention is directed to a coating composition formed from components comprising at least one carbamate functional material comprising at least one carbamate group blocked with a hydrolyzable silyl group, and at least one curing agent. Another embodiment of the present invention is directed to a coating composition formed from components comprising at least one carboxyl functional material comprising at least one carboxyl group blocked with a hydrolyzable silyl group, and at least one curing agent. Another embodiment of the present invention is directed to a coating composition formed from components comprising at least one amide functional material comprising at least one amide blocked with a hydrolyzable silyl group, and at least one curing agent. Other embodiments of the present invention are directed to substrates coated with the aforementioned cured compositions. Also provided are multi-component composite coatings which include a cured basecoat deposited from a pigmented coating composition and a cured topcoat deposited from a topcoating composition. The multi-component composite coatings of the invention provide highly scratch resistant color-plus-clearcoatings. Further embodiments of the present invention are directed to methods for improving scratch resistance of a substrate.

    摘要翻译： 由至少一种包含至少一个用可水解甲硅烷基封端的醇羟基的羟基官能非乙烯基材料形成的涂料组合物和至少一种固化剂由本发明提供。 本发明的另一个实施方案涉及由包含至少一种氨基甲酸酯官能材料的组分形成的涂料组合物，所述氨基甲酸酯官能材料包含至少一个被可水解甲硅烷基封端的氨基甲酸酯基团和至少一种固化剂。 本发明的另一个实施方案涉及由包含至少一种包含至少一个被可水解甲硅烷基封端的羧基的羧基官能材料和至少一种固化剂的组分形成的涂料组合物。 本发明的另一个实施方案涉及由包含至少一种酰胺官能材料的组分形成的涂料组合物，所述酰胺官能材料包含至少一个用可水解甲硅烷基封端的酰胺和至少一种固化剂。 本发明的其它实施方案涉及用上述固化组合物涂覆的基材。 还提供了多组分复合涂层，其包括由着色涂料组合物沉积的固化底涂层和从表面涂层组合物沉积的固化顶涂层。 本发明的多组分复合涂层提供高耐刮擦的彩色 - 透明涂层。 本发明的其它实施方案涉及用于改善基材的耐刮擦性的方法。

    Coating compositions comprising silyl blocked components, coating, coated substrates and methods related thereto
    5.
    发明授权
    Coating compositions comprising silyl blocked components, coating, coated substrates and methods related thereto 失效
    包含甲硅烷基封端组分，涂层，涂覆基材和与之有关的方法的涂料组合物

    公开(公告)号：US06635341B1

    公开(公告)日：2003-10-21

    申请号：US09629421

    申请日：2000-07-31

    申请人： Steven V. Barancyk ,  John W. Burgman ,  James B. O'Dywer ,  Laura A. Kiefer-Liptak ,  Michael Allen Mayo ,  Gregory J. McCollum ,  Shiryn Tyebjee

    发明人： Steven V. Barancyk ,  John W. Burgman ,  James B. O'Dywer ,  Laura A. Kiefer-Liptak ,  Michael Allen Mayo ,  Gregory J. McCollum ,  Shiryn Tyebjee

    IPC分类号： B32B516

    CPC分类号： C09D201/06 ,  C08G18/4692 ,  C08G18/792 ,  C09D167/00 ,  C09D175/04 ,  Y10T428/25 ,  Y10T428/251 ,  Y10T428/254 ,  Y10T428/2991 ,  Y10T428/2993 ,  Y10T428/2998 ,  Y10T428/31511 ,  Y10T428/31551 ,  C08L2666/28 ,  C08L2666/16

    摘要： Coating compositions formed from at least one hydroxyl functional non-vinyl material comprising at least one alcoholic hydroxyl group blocked with a hydrolyzable silyl group, and at least one curing agent are provided by the present invention. Another embodiment of the present invention is directed to a coating composition formed from components comprising at least one carbamate functional material comprising at least one carbamate group blocked with a hydrolyzable silyl group, and at least one curing agent. Another embodiment of the present invention is directed to a coating composition formed from components comprising at least one carboxyl functional material comprising at least one carboxyl group blocked with a hydrolyzable silyl group, and at least one curing agent. Another embodiment of the present invention is directed to a coating composition, formed from components comprising at least one amide functional material comprising at least one amide blocked with a hydrolyzable silyl group, and at least one curing agent. Other embodiments of the present invention are directed to substrates coated with the aforementioned cured compositions. Also provided are multi-component composite coatings which include a cured basecoat deposited from a pigmented coating composition and a cured topcoat deposited from a topcoating composition. The multi-component composite coatings of the invention provide highly scratch resistant color-plus-clearcoatings. Further embodiments of the present invention are directed to methods for improving scratch resistance of a substrate.

    摘要翻译： 由至少一种包含至少一个用可水解甲硅烷基封端的醇羟基的羟基官能非乙烯基材料形成的涂料组合物和至少一种固化剂由本发明提供。 本发明的另一个实施方案涉及由包含至少一种氨基甲酸酯官能材料的组分形成的涂料组合物，所述氨基甲酸酯官能材料包含至少一个被可水解甲硅烷基封端的氨基甲酸酯基团和至少一种固化剂。 本发明的另一个实施方案涉及由包含至少一种包含至少一个被可水解甲硅烷基封端的羧基的羧基官能材料和至少一种固化剂的组分形成的涂料组合物。 本发明的另一个实施方案涉及由包含至少一种酰胺官能材料的组分形成的涂料组合物，所述酰胺官能材料包含至少一个用可水解甲硅烷基封端的酰胺和至少一种固化剂。 本发明的其它实施方案涉及用上述固化组合物涂覆的基材。 还提供了多组分复合涂层，其包括由着色涂料组合物沉积的固化底涂层和从表面涂层组合物沉积的固化顶涂层。 本发明的多组分复合涂层提供高耐刮擦的彩色 - 透明涂层。 本发明的其它实施方案涉及用于改善基材的耐刮擦性的方法。

    Amide functional monomers and acrylic polymers with amide functionality
    6.
    发明授权
    Amide functional monomers and acrylic polymers with amide functionality 失效
    酰胺官能单体和具有酰胺官能团的丙烯酸聚合物

    公开(公告)号：US5859174A

    公开(公告)日：1999-01-12

    申请号：US681050

    申请日：1996-07-22

    申请人： Steven V. Barancyk ,  Neil D. McMurdie ,  James B. O'Dwyer

    发明人： Steven V. Barancyk ,  Neil D. McMurdie ,  James B. O'Dwyer

    IPC分类号： C07C235/06 ,  C08F20/36 ,  C08F18/00 ,  C08F20/54

    CPC分类号： C07C235/06 ,  C08F20/36

    摘要： Ethylenically unsaturated compounds are provided having Structure I and from which polymers with a plurality of groups of Structure II are derived. ##STR1## In Structures I and II, R.sub.1 is hydrogen or methyl, and R.sub.3 is hydrogen or lower alkyl having 1 to 4 carbon atoms, and when R.sub.3 is hydrogen and R.sub.2 has two carbon atoms R.sub.2 is methyl methylene. In Structure I, R.sub.2 and in Structure II R'.sub.2 is a divalent linking group having 2 to 20 carbon atoms. When R.sub.3 is hydrogen and R'.sub.2 has two carbon atoms, R'.sub.2 is methyl methylene. The compounds of Structure I may be used as monomers and reacted with other ethylenically unsaturated monomers via addition polymerization to arrive at the polymer with groups of Structure II.

    摘要翻译： 提供具有结构I的烯键式不饱和化合物，并从中得到具有多个结构II的基团的聚合物。 结构I和II，R 1是氢或甲基，R 3是氢或具有1至4个碳原子的低级烷基，当R 3是氢且R 2具有两个碳原子时，R 2是甲基亚甲基。 在结构I中，R 2和结构II中，R'2是具有2至20个碳原子的二价连接基团。 当R3是氢并且R'2具有两个碳原子时，R'2是甲基亚甲基。 结构I的化合物可以用作单体，并通过加成聚合与其它烯属不饱和单体反应，以结构II的基团得到聚合物。

    Curable film-forming compositions containing amide functional polymers
    7.
    发明授权
    Curable film-forming compositions containing amide functional polymers 失效
    含有酰胺官能聚合物的可固化成膜组合物

    公开(公告)号：US5780559A

    公开(公告)日：1998-07-14

    申请号：US681051

    申请日：1996-07-22

    申请人： Leigh-Ann Humbert ,  Daniel E. Rardon ,  Michael A. Mayo ,  Steven V. Barancyk ,  James B. O'Dwyer

    发明人： Leigh-Ann Humbert ,  Daniel E. Rardon ,  Michael A. Mayo ,  Steven V. Barancyk ,  James B. O'Dwyer

    IPC分类号： C08G18/38 ,  C08G18/62 ,  C08G18/66 ,  C08L61/20 ,  C09D133/06 ,  C09D133/26 ,  C09D201/02 ,  C08G18/00

    CPC分类号： C09D133/26 ,  C08G18/3823 ,  C08G18/3825 ,  C08G18/6216 ,  C08G18/6633 ,  C08G18/6666 ,  C09D133/062 ,  C09D201/02 ,  C08L61/20

    摘要： A film-forming composition is provided comprising: (i) an amide functional polymer, copolymer or oligomer selected from (a) acrylic polymers, (b) polyesters, (c) polyurethanes, (d) polyethers or (e) mixtures thereof; and (ii) an aminoplast crosslinking agent containing methylol and/or methylol ether groups. The acrylic polymers have a plurality of groups of at least one of the structures: ##STR1## wherein n is 0 or 1, R.sub.1 is hydrogen or methyl, R.sub.2 is a divalent linking group having about 1 to 30 carbon atoms when the group is of the first structure, or R.sub.2 is alkylene having about 2 to 13 carbon atoms when the group is of structure II, and R.sub.3 is hydrogen or lower alkyl having 1 to 4 carbon atoms. The (b), (c), and (d) polymers each have a plurality of terminal amide groups. The film-forming composition prior to curing has a theoretical hydroxyl value less than about 50 based on total resin solid weight of the film-forming composition, excluding any hydroxyl functionality associated with N-methylol groups. After curing, the film-forming composition exhibits a high level of acid etch resistance. The film forming composition can also be the clear film-forming composition with a base coat in a multi-component composite coating composition.

    摘要翻译： 提供一种成膜组合物，其包括：（i）酰胺官能聚合物，共聚物或低聚物，其选自（a）丙烯酸聚合物，（b）聚酯，（c）聚氨酯，（d）聚醚或（e）它们的混合物; 和（ii）含有羟甲基和/或羟甲基醚基团的氨基塑料交联剂。 丙烯酸类聚合物具有多个至少一个以下结构的基团：其中n为0或1，R 1为氢或甲基，R 2为具有约2个碳原子的二价连接基团 当该基团为第一结构时为1至30个碳原子，或当基团为结构II时，R 2为具有约2至13个碳原子的亚烷基，且R 3为氢或具有1至4个碳原子的低级烷基。 （b），（c）和（d）聚合物各自具有多个末端酰胺基团。 固化前的成膜组合物的理论羟值基于成膜组合物的总树脂固体重量小于约50，不包括与N-羟甲基相关的任何羟基官能团。 固化后，成膜组合物具有高水平的耐酸蚀性。 成膜组合物也可以是在多组分复合涂料组合物中具有底涂层的透明成膜组合物。

    CURABLE FILM-FORMING COMPOSITIONS CONTAINING COLLOIDAL SOLS HAVING IMPROVED APPEARANCE AND MAR AND SCRATCH RESISTANCE
    8.
    发明申请
    CURABLE FILM-FORMING COMPOSITIONS CONTAINING COLLOIDAL SOLS HAVING IMPROVED APPEARANCE AND MAR AND SCRATCH RESISTANCE 失效
    具有改善外观和耐刮擦性的胶体溶液的可固化成膜组合物

    公开(公告)号：US20090062461A1

    公开(公告)日：2009-03-05

    申请号：US11847427

    申请日：2007-08-30

    申请人： Steven V. Barancyk

    发明人： Steven V. Barancyk

    IPC分类号： C08G67/00

    CPC分类号： C08G65/336 ,  C08L33/00 ,  C08L71/02 ,  C08L2666/04

    摘要： Curable film-forming compositions comprising a film-forming resin and an organic sol of particles are provided. The sol of particles may be prepared by providing a suspension of particles in an aqueous medium; adding a first organic liquid compatible with the aqueous medium to form an admixture; reacting the particles with a first and a second modifying compound; adding a second organic liquid compatible with the liquid portion of the admixture wherein the second organic liquid is different from the first organic liquid; and maintaining the admixture at a temperature and pressure and for a time sufficient to substantially remove the water and the first organic liquid. The film-forming resin comprises an active hydrogen-functional polymer having low functionality; i.e., a functional group equivalent weight greater than 380 g/equivalent, and a crosslinking agent, yet surprisingly offers outstanding mar and scratch resistance.

    摘要翻译： 提供了包含成膜树脂和颗粒的有机溶胶的可成膜成膜组合物。 可以通过在水介质中提供颗粒的悬浮液来制备颗粒溶胶; 加入与水介质相容的第一有机液体以形成混合物; 使颗粒与第一和第二改性化合物反应; 添加与所述混合物的液体部分相容的第二有机液体，其中所述第二有机液体不同于所述第一有机液体; 并将混合物在温度和压力下保持足够的时间以基本上除去水和第一有机液体。 成膜树脂包含具有低官能度的活性氢官能聚合物; 即大于380g /当量的官能团当量，以及交联剂，令人惊奇的是具有优异的耐擦伤性和耐擦伤性。