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    HYDROGENATION CATALYST AND METHOD FOR PRODUCING SAME
    73.
    发明申请
    HYDROGENATION CATALYST AND METHOD FOR PRODUCING SAME 有权
    氢化催化剂及其生产方法

    公开(公告)号：US20140243192A1

    公开(公告)日：2014-08-28

    申请号：US14349105

    申请日：2012-10-22

    申请人： JGC CATALYSTS AND CHEMICALS LTD.

    发明人： Kenji Yamane ,  Kouichi Ohama ,  Shogo Tagawa

    IPC分类号： B01J27/19

    CPC分类号： B01J27/19 ,  B01J27/16 ,  B01J31/121 ,  B01J35/1019 ,  B01J35/1042 ,  B01J35/1047 ,  B01J35/1061 ,  B01J35/1085 ,  B01J35/109 ,  B01J37/0203 ,  B01J37/024 ,  B01J37/033 ,  B01J37/28 ,  C10G45/04 ,  C10G2300/201

    摘要： A hydrotreating catalyst includes a hydrogenation active metal supported on a alumina-phosphorus support and satisfies: a specific surface area being 100 m2/g or more; a total pore volume measured by mercury intrusion being in a range 0.80-1.50 ml/g; a maximum value of pore distribution being present in a pore diameter range 10-30 nm; a ratio of a pore volume of pores with a pore diameter within a range of ±2 nm of a pore diameter at the maximum value to a pore volume of pores with a pore diameter in a range 5-100 nm being 0.40 or less; a pressure capacity being 10 N/mm or more; 0.4-10.0 mass % of phosphorus being contained in the catalyst in terms of P2O5 concentration based on a total amount of the catalyst; and a hydrogenation active metal being at least one metal selected from metals of VIA and VIII groups of the periodic table.

    摘要翻译： 加氢处理催化剂包括负载在氧化铝 - 磷载体上的氢化活性金属，并且满足：比表面积为100m 2 / g以上; 通过水银侵入测量的总孔体积在0.80-1.50ml / g的范围内; 孔分布的最大值存在于10-30nm的孔径范围内; 孔直径在最大值的孔径±2nm范围内的孔的孔体积与孔径在5-100nm范围内的孔的孔体积的比为0.40以下; 压力容量为10N / mm以上; 以催化剂总量计，P2O5浓度中催化剂中含有0.4-10.0质量％的磷; 和加氢活性金属是选自元素周期表的VIA和VIII族金属中的至少一种金属。

    HIGH SEVERITY HYDROPROCESSING INTERSTITIAL METAL HYDRIDE CATALYSTS AND ASSOCIATED PROCESSES
    77.
    发明申请
    HIGH SEVERITY HYDROPROCESSING INTERSTITIAL METAL HYDRIDE CATALYSTS AND ASSOCIATED PROCESSES 审中-公开
    高含量水解间接金属氢化物催化剂及相关工艺

    公开(公告)号：US20110119993A1

    公开(公告)日：2011-05-26

    申请号：US12948595

    申请日：2010-11-17

    申请人： Faiz Pourarian ,  Marc A. Portnoff ,  David A. Purta ,  Margaret A. Nasta ,  Jingfeng Zhang

    发明人： Faiz Pourarian ,  Marc A. Portnoff ,  David A. Purta ,  Margaret A. Nasta ,  Jingfeng Zhang

    IPC分类号： C10L1/00 ,  B01J21/06 ,  B01J21/08

    CPC分类号： B01J31/121 ,  B01J23/83 ,  B01J35/002 ,  B01J37/0009 ,  B01J37/0036 ,  B01J37/18 ,  C10G45/04 ,  C22C16/00 ,  C22C28/00

    摘要： The present invention relates to the processing of hydrocarbon-containing feedstreams in the presence of an interstitial metal hydride containing catalyst and hydrogen at process conditions of at least 400 psig pressure and temperatures of at least 200° C. These processes use interstitial metal hydrides that possess significant hydrogen capacities and high hydrogen kinetics rate properties. The catalysts and processes of the present invention may be used with or without radio frequency or microwave energy and are preferably run under conditions of high hydrogen partial pressure above about 350 psia. The catalysts and processes of the present invention can improve overall hydrogenation, product conversion, as well as sulfur reduction in hydrocarbon feedstreams as compared to processes of the prior art operated under similar conditions.

    摘要翻译： 本发明涉及在至少400psig压力和至少200℃的温度的工艺条件下，在含有间隙金属氢化物的催化剂和氢气存在下，含烃进料流的加工。这些方法使用间隙金属氢化物，其具有 显着的氢气容量和高氢动力学特性。 本发明的催化剂和方法可以使用或不使用射频或微波能量，并且优选在高于约350psia的高氢分压的条件下运行。 与在类似条件下操作的现有技术的方法相比，本发明的催化剂和方法可以改进烃类进料流中的总体氢化，产物转化以及硫的还原。

    PROCESS FOR CONVERTING ETHANE INTO LIQUID ALKANE MIXTURES
    78.
    发明申请
    PROCESS FOR CONVERTING ETHANE INTO LIQUID ALKANE MIXTURES 审中-公开
    将乙醇转化成液体醇混合物的方法

    公开(公告)号：US20110071331A1

    公开(公告)日：2011-03-24

    申请号：US12451951

    申请日：2008-06-10

    申请人： Jean-Marie Basset ,  Sudhakar Chakka ,  Mostafa Taoufik ,  Jean Thivolle-Cazat

    发明人： Jean-Marie Basset ,  Sudhakar Chakka ,  Mostafa Taoufik ,  Jean Thivolle-Cazat

    IPC分类号： C07C2/00

    CPC分类号： C10L3/10 ,  B01J21/04 ,  B01J21/08 ,  B01J31/121 ,  B01J2531/58 ,  B01J2531/66 ,  C07C2/76 ,  C07C6/10 ,  C07C9/00 ,  C07C2521/04 ,  C07C2531/12 ,  C10G50/00 ,  C10G2300/1025 ,  C10G2300/703 ,  C07C9/06

    摘要： The invention relates to a process for converting ethane into liquid mixture of (C4+) alkanes having 4 carbon atoms and more, preferably (C5+) alkanes having 5 carbon atoms and more. The process comprises a stage (1) comprising simultaneous ethane self- and cross-metathesis reactions carried out by contacting ethane with a metal catalyst (C1) capable of producing, in contact with alkane, reactions involving the splitting and recombining of C—C and/or C—H and/or C-metal bonds, so as to form a reaction mixture (MI) comprising methane and a mixture of the (C4+), preferably the (C5+) alkanes, a stage (2) comprising separating and isolating methane from the reaction mixture (MI), a stage (3) comprising a non-oxidative methane coupling reaction carried out by contacting the methane thus isolated with a metal catalyst (C2) capable of producing, in contact with alkane, reactions involving the splitting and recombining of C—C and/or C—H and/or C-metal bonds, said catalyst (C2) being identical to or different from the catalyst (C1), so as to form a mixture (M2) comprising ethane and hydrogen, optionally a stage (4) comprising separating and isolating ethane from the mixture (M2), a stage (5) comprising recycling the ethane thus isolated or the mixture (M2) into stage (1) for going on with the simultaneous ethane self- and cross-metathesis reactions and continuing forming said reaction mixture (MI), and a stage (6) comprising separating and isolating.

    摘要翻译： 本发明涉及一种将乙烷转化成具有4个碳原子的（C 4+）烷烃和更多的（C 5+）烷烃，具有5个碳原子和更多的（C 5+）烷烃的液体混合物的方法。 该方法包括阶段（1），其包括同时进行的乙烷自交联和交叉复分解反应，其通过使乙烷与能够与烷烃接触的金属催化剂（C1）接触进行，所述反应涉及C-C的分解和重组以及 /或C-H和/或C - 金属键，以形成包含甲烷和（C4 +），优选（C5 +）烷烃的混合物的反应混合物（MI），包括分离和分离的级（2） 来自反应混合物（MI）的甲烷，包含非氧化性甲烷偶联反应的阶段（3），其通过使如此分离的甲烷与能够与烷烃接触的金属催化剂（C2）接触涉及分裂的反应 和C-C和/或C-H和/或C-金属键的重组，所述催化剂（C2）与催化剂（C1）相同或不同，从而形成包含乙烷和氢的混合物（M2） ，任选地包括从所述分离和分离乙烷的阶段（4） 混合物（M2），阶段（5），其包括将如此分离的乙烷或混合物（M2）循环到阶段（1）中，以进行同时进行的乙烷自交联和交叉复分解反应并连续形成所述反应混合物（MI） ，以及包括分离和分离的阶段（6）。

    PROCESS FOR MANUFACTURING NEOHEXENE
    79.
    发明申请
    PROCESS FOR MANUFACTURING NEOHEXENE 失效
    制造NEOHEXENE的工艺

    公开(公告)号：US20100030003A1

    公开(公告)日：2010-02-04

    申请号：US12448216

    申请日：2007-12-11

    申请人： Jean-Marie Basset ,  Francois Stoffelbach ,  Mostafa Taoufik ,  Jean Thivolle-Cazat

    发明人： Jean-Marie Basset ,  Francois Stoffelbach ,  Mostafa Taoufik ,  Jean Thivolle-Cazat

    IPC分类号： C07C6/00

    CPC分类号： C10L1/06 ,  B01J21/04 ,  B01J31/121 ,  B01J37/0209 ,  B01J2531/66 ,  C07C6/04 ,  C07C2521/04 ,  C07C2531/12 ,  C07C11/107

    摘要： The present invention relates to a process for manufacturing neohexene, comprising contacting isobutene with a supported catalyst comprising a tungsten compound chosen from tungsten hydrides, organometallic tungsten compounds and organometallic tungsten hydrides, and a support comprising an oxide of aluminium, so as to form a reaction mixture comprising neohexene, and preferably separating neohexene from the reaction mixture, so as to isolate it. The contacting leads to the direct production of neohexene, in particular in a single (reaction) stage and with a high molar selectivity for neohexene. The contacting can be performed at a temperature of 50 to 600° C., under a total absolute pressure of 0.01 to 100 MPa.

    摘要翻译： 本发明涉及一种制备新己烯的方法，包括使异丁烯与包含选自氢化钨，有机金属钨化合物和有机金属氢化钨的钨化合物的负载催化剂和包含铝氧化物的载体接触，以形成反应 包含新己烯的混合物，优选从反应混合物中分离新己烯，以便将其分离。 接触导致新己烯的直接生产，特别是在单一（反应）阶段和对新己烯的高摩尔选择性。 接触可以在50〜600℃的温度下，在0.01〜100MPa的绝对压力下进行。

    Process for manufacturing alkanes by reacting other alkanes with methane
    80.
    发明授权
    Process for manufacturing alkanes by reacting other alkanes with methane 失效
    通过使其他烷烃与甲烷反应制备烷烃的方法

    公开(公告)号：US07378564B2

    公开(公告)日：2008-05-27

    申请号：US10502845

    申请日：2003-01-22

    申请人： Jean-Marie Basset ,  Christophe Coperet ,  Richard Pardy ,  Daravong Soulivong ,  John Glenn Sunley ,  Jean Thivolle-Cazat

    发明人： Jean-Marie Basset ,  Christophe Coperet ,  Richard Pardy ,  Daravong Soulivong ,  John Glenn Sunley ,  Jean Thivolle-Cazat

    IPC分类号： C07C6/08

    CPC分类号： C07C6/10 ,  B01J21/08 ,  B01J31/121 ,  B01J37/0209 ,  C07C2531/12 ,  Y10S585/943

    摘要： The present invention relates to a process for the manufacture of alkanes comprising a catalytic reaction resulting from contacting methane with at least one other starting alkane (I) in the presence of a metal compound (C) capable of catalysing a reaction for the splitting and/or recombination of a carbon-carbon bond and/or of a carbon-hydrogen bond and/or of a carbon-metal bond, which catalytic reaction results in the formation of at least one final alkane (II) having a number of carbon atoms equal to or greater than (2). In the process, the contacting operation is carried out under a methane partial pressure equal to or greater than 0.1 MPa, preferably in the range from 0.1 to 100 MPa. The metal compound (C) can be chosen from metal compounds supported on and dispersed over a solid support, metal compounds supported on and grafted to a solid support and non-supported metal compounds. Under these conditions, it was found that the yield of the catalytic reaction was improved, and that the catalytic stability and activity of the metal compound (C) over timer were greatly enhanced.

    摘要翻译： 本发明涉及一种制备烷烃的方法，其包括由甲烷与至少一种其它起始烷烃（I）在能够催化分解和/或反应的反应的金属化合物（C）存在下使甲烷接触而产生的催化反应， 或碳 - 碳键和/或碳 - 氢键和/或碳 - 金属键的重组，该催化反应导致至少一个具有多个碳原子的最终烷烃（II）的形成相等 至（2）以上。 在该过程中，接触操作在等于或大于0.1MPa，优选在0.1至100MPa范围内的甲烷分压下进行。 金属化合物（C）可以选自负载在固体载体上并分散在固体载体上的金属化合物，负载在和接枝到固体载体上的金属化合物和非负载的金属化合物。 在这些条件下，发现催化反应的产率提高，金属化合物（C）超过定时器的催化稳定性和活性大大提高。